Estimating the average time for inter-continental transport of air pollutants

被引:17
作者
Liu, JF [1 ]
Mauzerall, DL [1 ]
机构
[1] Princeton Univ, Woodrow Wilson Sch Publ & Int Affairs, Princeton, NJ 08540 USA
关键词
D O I
10.1029/2005GL022619
中图分类号
P [天文学、地球科学];
学科分类号
07 ;
摘要
We estimate the average time required for intercontinental transport of atmospheric tracers based on simulations with the global chemical tracer model MOZART-2 driven with NCEP meteorology. We represent the average transport time by a ratio of the concentration of two tracers with different lifetimes. We find that average transport times increase with tracer lifetimes. With tracers of 1- and 2-week lifetimes the average transport time from East Asia (EA) to the surface of western North America (NA) in April is 2-3 weeks, approximately a half week longer than transport from NA to western Europe (EU) and from EU to EA. We develop an 'equivalent circulation' method to estimate a timescale which has little dependence on tracer lifetimes and obtain similar results to those obtained with short-lived tracers. Our findings show that average intercontinental transport times, even for tracers with short lifetimes, are on average 1- 2 weeks longer than rapid transport observed in plumes.
引用
收藏
页码:1 / 4
页数:4
相关论文
共 14 条
[1]   Atmospheric organochlorine pesticides in the western Canadian Arctic: Evidence of transpacific transport [J].
Bailey, R ;
Barrie, LA ;
Halsall, CJ ;
Fellin, P ;
Muir, DCG .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2000, 105 (D9) :11805-11811
[2]   AGE AS A DIAGNOSTIC OF STRATOSPHERIC TRANSPORT [J].
HALL, TM ;
PLUMB, RA .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 1994, 99 (D1) :1059-1070
[3]   Springtime trans-Pacific atmospheric transport from east Asia: A transit-time probability density function approach [J].
Holzer, M ;
McKendry, IG ;
Jaffe, DA .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2003, 108 (D22)
[4]   A global simulation of tropospheric ozone and related tracers: Description and evaluation of MOZART, version 2 [J].
Horowitz, LW ;
Walters, S ;
Mauzerall, DL ;
Emmons, LK ;
Rasch, PJ ;
Granier, C ;
Tie, XX ;
Lamarque, JF ;
Schultz, MG ;
Tyndall, GS ;
Orlando, JJ ;
Brasseur, GP .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2003, 108 (D24)
[5]   Asian dust events of April 1998 [J].
Husar, RB ;
Tratt, DM ;
Schichtel, BA ;
Falke, SR ;
Li, F ;
Jaffe, D ;
Gassó, S ;
Gill, T ;
Laulainen, NS ;
Lu, F ;
Reheis, MC ;
Chun, Y ;
Westphal, D ;
Holben, BN ;
Gueymard, C ;
McKendry, I ;
Kuring, N ;
Feldman, GC ;
McClain, C ;
Frouin, RJ ;
Merrill, J ;
DuBois, D ;
Vignola, F ;
Murayama, T ;
Nickovic, S ;
Wilson, WE ;
Sassen, K ;
Sugimoto, N ;
Malm, WC .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2001, 106 (D16) :18317-18330
[6]   Six 'new' episodes of trans-Pacific transport of air pollutants [J].
Jaffe, D ;
McKendry, I ;
Anderson, T ;
Price, H .
ATMOSPHERIC ENVIRONMENT, 2003, 37 (03) :391-404
[7]   Transport of Asian air pollution to North America [J].
Jaffe, D ;
Anderson, T ;
Covert, D ;
Kotchenruther, R ;
Trost, B ;
Danielson, J ;
Simpson, W ;
Berntsen, T ;
Karlsdottir, S ;
Blake, D ;
Harris, J ;
Carmichael, G ;
Uno, I .
GEOPHYSICAL RESEARCH LETTERS, 1999, 26 (06) :711-714
[8]   Analysis of seasonal and interannual variability in transpacific transport [J].
Liu, JF ;
Mauzerall, DL ;
Horowitz, LW .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2005, 110 (D4) :1-17
[9]   Photochemistry in biomass burning plumes and implications for tropospheric ozone over the tropical South Atlantic [J].
Mauzerall, DL ;
Logan, JA ;
Jacob, DJ ;
Anderson, BE ;
Blake, DR ;
Bradshaw, JD ;
Heikes, B ;
Sachse, GW ;
Singh, H ;
Talbot, B .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 1998, 103 (D7) :8401-8423
[10]   Hydrocarbon ratios during PEM-WEST A: A model perspective [J].
McKeen, SA ;
Liu, SC ;
Hsie, EY ;
Lin, X ;
Bradshaw, JD ;
Smyth, S ;
Gregory, GL ;
Blake, DR .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 1996, 101 (D1) :2087-2109