Strong velocity effects in collisions of He+ with fullerenes

被引:79
作者
Schlathölter, T [1 ]
Hadjar, O [1 ]
Hoekstra, R [1 ]
Morgenstern, R [1 ]
机构
[1] Univ Groningen, KVI Atom Phys, NL-9747 AA Groningen, Netherlands
关键词
D O I
10.1103/PhysRevLett.82.73
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We have studied fragmentation and ionization of C-60 by He+ impact over a velocity range from 0.1 to 1 a.u. where a transition from vibrational to electronic excitation is predicted. With increasing velocity we observe a strong decrease of evaporative processes (C-60-2m(r+) peaks) and a linearly increasing yield of small fragments (C-n(+), n < 15). Apparently direct vibrational excitation leads preferentially to evaporation, whereas electronic excitation is responsible for multifragmentation. In the intermediate range we find indications for a "transparency window" similar to that predicted recently in simulations of Na-9(+)-He collisions. [S0031-9007(98)08105-8].
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页码:73 / 76
页数:4
相关论文
共 32 条
[1]   EMPIRICAL POTENTIAL FOR HYDROCARBONS FOR USE IN SIMULATING THE CHEMICAL VAPOR-DEPOSITION OF DIAMOND FILMS [J].
BRENNER, DW .
PHYSICAL REVIEW B, 1990, 42 (15) :9458-9471
[2]   Analysis of collision induced dissociation of Na-2(+) molecular ions [J].
Brenot, JC ;
Dunet, H ;
Fayeton, JA ;
Barat, M ;
Winter, M .
PHYSICAL REVIEW LETTERS, 1996, 77 (07) :1246-1249
[3]   Internal energy dependence of the fragmentation patterns of C-60 and C-60(+) [J].
Campbell, EEB ;
Raz, T ;
Levine, RD .
CHEMICAL PHYSICS LETTERS, 1996, 253 (3-4) :261-267
[4]   Ionization and fragmentation of C-60 by highly charged, high-energy xenon ions [J].
Cheng, S ;
Berry, HG ;
Dunford, RW ;
Esbensen, H ;
Gemmell, DS ;
Kanter, EP ;
LeBrun, T ;
Bauer, W .
PHYSICAL REVIEW A, 1996, 54 (04) :3182-3194
[5]   ELECTRON-IMPACT IONIZATION OF C-60 [J].
DUNSER, B ;
LEZIUS, M ;
SCHEIER, P ;
DEUTSCH, H ;
MARK, TD .
PHYSICAL REVIEW LETTERS, 1995, 74 (17) :3364-3367
[6]   A THEORETICAL-STUDY OF THE C-2 FRAGMENTATION ENERGY OF C-60 AND C-70 [J].
ECKHOFF, WC ;
SCUSERIA, GE .
CHEMICAL PHYSICS LETTERS, 1993, 216 (3-6) :399-404
[7]   Fragmentation of fullerenes in collisions with atomic and molecular targets [J].
Ehlich, R ;
Westerburg, M ;
Campbell, EEB .
JOURNAL OF CHEMICAL PHYSICS, 1996, 104 (05) :1900-1911
[8]   COLLISIONAL DYNAMICS OF C-60 WITH NOBLE-GAS-ATOMS STUDIED BY MOLECULAR-DYNAMICS WITH EMPIRICAL 2-BODY AND 3-BODY FORCES [J].
EHLICH, R ;
CAMPBELL, EEB ;
KNOSPE, O ;
SCHMIDT, R .
ZEITSCHRIFT FUR PHYSIK D-ATOMS MOLECULES AND CLUSTERS, 1993, 28 (02) :153-161
[9]   Molecular dynamics studies of inelastic scattering and fragmentation in collisions of C60 with rare-gas atoms [J].
Ehlich, R ;
Knospe, O ;
Schmidt, R .
JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS, 1997, 30 (23) :5429-5449
[10]   FRICTION PARAMETER OF AN ION NEAR A METAL-SURFACE [J].
FERRELL, TL ;
ECHENIQUE, PM ;
RITCHIE, RH .
SOLID STATE COMMUNICATIONS, 1979, 32 (05) :419-422