A Numerical Model for Predicting Gas Diffusion Layer Failure in Proton Exchange Membrane Fuel Cells

被引:37
作者
Yi, Peiyun [1 ]
Peng, Linfa [1 ]
Lai, Xinmin [1 ]
Ni, Jun [2 ]
机构
[1] Shanghai Jiao Tong Univ, State Key Lab Mech Syst & Vibrat, Shanghai 200240, Peoples R China
[2] Univ Michigan, Dept Mech Engn, Ann Arbor, MI 48109 USA
来源
JOURNAL OF FUEL CELL SCIENCE AND TECHNOLOGY | 2011年 / 8卷 / 01期
基金
中国国家自然科学基金;
关键词
proton exchange membrane fuel cell; gas diffusion layer; assembly pressure; failure criterion; prediction model; ELECTRICAL CONTACT RESISTANCE; BIPOLAR PLATE; PERFORMANCE; COMPRESSION; STRENGTH;
D O I
10.1115/1.4002312
中图分类号
O646 [电化学、电解、磁化学];
学科分类号
081704 ;
摘要
Gas diffusion layer (GDL) is one of the critical components in proton exchange membrane fuel cells (PEMFCs) and plays several important roles, such as structural support, reactants permeation, water removal, electrons, and heat conduction. The assembly pressure on bipolar plate is an important factor that affects the performance of PEMFC stack. Not enough assembly pressure leads to leakage of fuels and high contact resistance. Too much pressure, on the other hand, results in damage to the GDL, which increases the GDL Ohmic resistance and interfacial contact resistance, and in turn influences the reactant transport and water removal. The objective of the present study is to develop a numerical model to predict the onset of GDL failure and obtain the maximum assembly pressure on bipolar plate. Composite micromechanical model is applied to calculate the effective elastic properties of GDL; strength failure criterion is established to judge GDL damage with the stress distribution; finite element method model is developed to show the failure zone and the failure propagation in GDL combining the estimated elastic properties and strength failure criterion. Toray TGP-H-060 carbon paper is introduced as a numerical example and the numerical results show good agreements with experimental results. This numerical prediction model is beneficial to understand the basic mechanism of GDL failure and helpful to guide the assembling of PEMFC stack. [DOI:10.1115/1.4002312]
引用
收藏
页数:10
相关论文
共 35 条
[1]  
*AB INC, ABAQUS V6 7 US MAN
[2]   THE USE OF TENSORS TO DESCRIBE AND PREDICT FIBER ORIENTATION IN SHORT FIBER COMPOSITES [J].
ADVANI, SG ;
TUCKER, CL .
JOURNAL OF RHEOLOGY, 1987, 31 (08) :751-784
[3]  
[Anonymous], 2004, Fuel Cell Handbook, V7
[4]  
ASTM International, 2008, D3039 ASTM
[5]   Effect of compression on liquid water transport and microstructure of PEMFC gas diffusion layers [J].
Bazylak, A. ;
Sinton, D. ;
Liu, Z. -S. ;
Djilali, N. .
JOURNAL OF POWER SOURCES, 2007, 163 (02) :784-792
[6]   A SIMPLE ILLUSTRATION OF STRUCTURE-PROPERTIES RELATIONSHIPS FOR SHORT FIBER-REINFORCED THERMOPLASTICS [J].
DOSHI, SR ;
CHARRIER, JM .
POLYMER COMPOSITES, 1989, 10 (01) :28-38
[7]   Characterization of PEMFCs gas diffusion layers properties [J].
Escribano, Sylvie ;
Blachot, Jean-Francois ;
Etheve, Jeremy ;
Morin, Arnaud ;
Mosdale, Renaut .
JOURNAL OF POWER SOURCES, 2006, 156 (01) :8-13
[8]  
HATTUM FWJ, 1999, POLYM COMPOSITE, V20, P524
[9]   Two-phase flow model of the cathode of PEM fuel cells using interdigitated flow fields [J].
He, WS ;
Yi, JS ;
Nguyen, TV .
AICHE JOURNAL, 2000, 46 (10) :2053-2064
[10]  
Hedgepeth JM., 1967, J Compos Mater, V1, P294, DOI DOI 10.1177/002199836700100305