Competition between sequential and direct paths in a two-photon transition

被引:59
作者
Chatel, B [1 ]
Degert, J [1 ]
Stock, S [1 ]
Girard, B [1 ]
机构
[1] Univ Toulouse 3, IRSAMC, CNRS,UMR 5589, Lab Collis Agregats & React, F-31062 Toulouse, France
来源
PHYSICAL REVIEW A | 2003年 / 68卷 / 04期
关键词
D O I
10.1103/PhysRevA.68.041402
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
Two-photon excitation of a quantum ladder system by a chirped pulse leads to interferences in the excited-state population, due to the phase differences between direct and sequential paths. First, based on an analytical approach, we separate and discuss the features of the contributions arising from these two paths. Then interferences with two intermediate levels are observed experimentally in atomic sodium vapor. Interplay between the two sequential paths leads to strongly contrasted oscillations and a great enhancement of the transition probability for some values of the chirp.
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页数:4
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共 40 条
[1]   Coherent control by a single phase shaped femtosecond laser pulse [J].
Assion, A ;
Baumert, T ;
Helbing, J ;
Seyfried, V ;
Gerber, G .
CHEMICAL PHYSICS LETTERS, 1996, 259 (5-6) :488-494
[2]   Simultaneous control of time-dependent population transfer dynamics and wave-packet quantum interferences in Li2by shaped ultrafast pulses [J].
Ballard, Joshua B. ;
Stauffer, Hans U. ;
Mirowski, Elizabeth ;
Leone, Stephen R. .
Physical Review A - Atomic, Molecular, and Optical Physics, 2002, 66 (04) :434021-434027
[3]   INTERFERENCE IN CLIMBING A QUANTUM LADDER SYSTEM WITH FREQUENCY-CHIRPED LASER-PULSES [J].
BALLING, P ;
MAAS, DJ ;
NOORDAM, LD .
PHYSICAL REVIEW A, 1994, 50 (05) :4276-4285
[4]   MULTIPHOTON ABSORPTION VIA CHIRPED-PULSE ADIABATIC PASSAGE - DYNAMICS WITHIN THE EXCITED-STATE MANIFOLDS [J].
BAND, YB .
PHYSICAL REVIEW A, 1994, 50 (06) :5046-5050
[5]   Feasibility study to create a polychromatic guidestar in atomic sodium [J].
Biegert, J ;
Diels, JC .
PHYSICAL REVIEW A, 2003, 67 (04) :11
[6]   Bichromatic two-photon coherent excitation of sodium to provide a dual-wavelength guidestar [J].
Biegert, J ;
Diels, JC ;
Milonni, PW .
OPTICS LETTERS, 2000, 25 (10) :683-685
[7]   EXPERIMENTAL EVIDENCE OF 2-PHOTON TRANSITION WITHOUT DOPPLER BROADENING [J].
BIRABEN, F ;
CAGNAC, B ;
GRYNBERG, G .
PHYSICAL REVIEW LETTERS, 1974, 32 (12) :643-645
[8]   RESONANT ENHANCEMENT OF 2-PHOTON ABSORPTION IN SODIUM VAPOR [J].
BJORKHOLM, JE ;
LIAO, PF .
PHYSICAL REVIEW LETTERS, 1974, 33 (03) :128-131
[9]   EFFICIENT POPULATION TRANSFER IN A 3-LEVEL LADDER SYSTEM BY FREQUENCY-SWEPT ULTRASHORT LASER-PULSES [J].
BROERS, B ;
VANDENHEUVELL, HBV ;
NOORDAM, LD .
PHYSICAL REVIEW LETTERS, 1992, 69 (14) :2062-2065
[10]   Selective excitation of diatomic molecules by chirped laser pulses [J].
Chang, BY ;
Solá, IR ;
Malinovsky, VS ;
Santamaría, J .
JOURNAL OF CHEMICAL PHYSICS, 2000, 113 (12) :4901-4911