Non-equilibrium magnetization dynamics in the Fe8 single-molecule magnet induced by high-intensity microwave radiation

被引:20
作者
Bal, M [1 ]
Friedman, JR
Suzuki, Y
Rumberger, EM
Hendrickson, DN
Avraham, N
Myasoedov, Y
Shtrikman, H
Zeldov, E
机构
[1] Amherst Coll, Dept Phys, Amherst, MA 01002 USA
[2] CUNY City Coll, Dept Phys, New York, NY 10031 USA
[3] Univ Calif San Diego, Dept Chem & Biochem, La Jolla, CA 92093 USA
[4] Weizmann Inst Sci, Dept Condensed Matter Phys, IL-76100 Rehovot, Israel
来源
EUROPHYSICS LETTERS | 2005年 / 71卷 / 01期
关键词
D O I
10.1209/epl/i2005-10069-3
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
Resonant microwave radiation applied to a single crystal of the molecular magnet Fe-8 induces dramatic changes in the sample's magnetization. Transitions between excited states are found even though at the nominal system temperature these levels have negligible population. We find evidence that the sample heats significantly when the resonance condition is met. In addition, heating is observed after a short pulse of intense radiation has been turned off, indicating that the spin system is out of equilibrium with the lattice.
引用
收藏
页码:110 / 116
页数:7
相关论文
共 20 条
[1]   Microwave absorption and magnetization tunneling in Mn12-acetate molecular clusters -: art. no. 220402 [J].
Amigó, R ;
Hernandez, JM ;
García-Santiago, A ;
Tejada, J .
PHYSICAL REVIEW B, 2003, 67 (22)
[2]   Photon-induced magnetization reversal in the Fe8 single-molecule magnet -: art. no. 100408 [J].
Bal, M ;
Friedman, JR ;
Suzuki, Y ;
Mertes, KM ;
Rumberger, EM ;
Hendrickson, DN ;
Myasoedov, Y ;
Shtrikman, H ;
Avraham, N ;
Zeldov, E .
PHYSICAL REVIEW B, 2004, 70 (10) :100408-1
[3]  
Barra AL, 2000, CHEM-EUR J, V6, P1608, DOI 10.1002/(SICI)1521-3765(20000502)6:9<1608::AID-CHEM1608>3.3.CO
[4]  
2-#
[5]   Monolayer growth modes of Re and Nb on 4H-SiC(0001) and 4H-SiC(000(1)over-bar) [J].
Bryant, KW ;
Bozack, MJ .
JOURNAL OF APPLIED PHYSICS, 2005, 97 (02)
[6]   Neutron spectroscopy for the magnetic anisotropy of molecular clusters [J].
Caciuffo, R ;
Amoretti, G ;
Murani, A ;
Sessoli, R ;
Caneschi, A ;
Gatteschi, D .
PHYSICAL REVIEW LETTERS, 1998, 81 (21) :4744-4747
[7]   Quantum superposition of high spin states in the single molecule magnet Ni4 -: art. no. 157202 [J].
del Barco, E ;
Kent, AD ;
Yang, EC ;
Hendrickson, DN .
PHYSICAL REVIEW LETTERS, 2004, 93 (15) :157202-1
[8]  
DOUGLAS LM, 1966, PHYS REV, V141, P576
[9]  
Friedman J. R., 2003, EXPLORING QUANTUM CL, P179
[10]   Macroscopic measurement of resonant magnetization tunneling in high-spin molecules [J].
Friedman, JR ;
Sarachik, MP ;
Tejada, J ;
Ziolo, R .
PHYSICAL REVIEW LETTERS, 1996, 76 (20) :3830-3833