Subdiffraction far-field imaging of luminescent single-walled carbon nanotubes

被引:34
作者
Cognet, Laurent [1 ,2 ,3 ]
Tsyboulski, Dmitri A. [1 ,2 ]
Weisman, R. Bruce [1 ,2 ]
机构
[1] Rice Univ, Dept Chem, Richard E Smalley Inst Nanoscale Sci & Technol, Houston, TX 77005 USA
[2] Rice Univ, Ctr Biol & Environm Nanotechnol, Houston, TX 77005 USA
[3] Univ Bordeaux 1, Ctr Phys Mol Opt & Hertzienne, F-33405 Talence, France
关键词
D O I
10.1021/nl0725300
中图分类号
O6 [化学];
学科分类号
0703 [化学];
摘要
Far-field near-infrared fluorescence microscopy of single-walled carbon nanotubes (SWNTs) has been hampered by the diffraction limit to resolution. A new analysis method is presented that allows subwavelength (lambda/10) mapping of single-molecule chemical reaction sites on semiconducting SWNTs, enabling precise localization of excitonic luminescence regions along the nanotube axis through a nonperturbing, far-field optical measurement. This method is applied to reveal the subdiffraction lengths, curvatures, and defects of luminescent SWNTs in unprecedented detail.
引用
收藏
页码:749 / 753
页数:5
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