Influence of nitrogen content on the acid-base properties of aluminophosphate oxynitrides

被引:61
作者
Massinon, A
Odriozola, JA
Bastians, P
Conanec, R
Marchand, R
Laurent, Y
Grange, P
机构
[1] UNIV CATHOLIQUE LOUVAIN, UNITE CATALYSE & CHIM MAT DIVISES, B-1348 LOUVAIN, BELGIUM
[2] UNIV SEVILLA, DEPT QUIM INORGAN, E-41071 SEVILLE, SPAIN
[3] UNIV RENNES 1, URA 1496 CNRS, LAB CHIM MAT, F-35042 RENNES, FRANCE
关键词
acid-base properties; aluminophosphate oxynitrides; Knoevenagel condensation; nitrogen;
D O I
10.1016/0926-860X(95)00255-3
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Novel basic catalysts with high specific surface areas have been synthesized by activation under ammonia of an aluminophosphate oxide precursor. The nitrogen content as well as the acid-base properties depend on both time and temperature of nitridation. The conversion and reaction rate in Knoevenagel condensation are related to the nitrogen content.
引用
收藏
页码:9 / 23
页数:15
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