Emission inventory of anthropogenic air pollutants and VOC species in the Yangtze River Delta region, China

被引:298
作者
Huang, C. [1 ]
Chen, C. H. [1 ]
Li, L. [1 ]
Cheng, Z. [2 ]
Wang, H. L. [1 ]
Huang, H. Y. [1 ]
Streets, D. G. [3 ]
Wang, Y. J. [4 ]
Zhang, G. F. [1 ]
Chen, Y. R. [1 ]
机构
[1] Shanghai Acad Environm Sci, Shanghai 200233, Peoples R China
[2] Tsinghua Univ, Dept Environm Sci & Engn, Beijing 100084, Peoples R China
[3] Argonne Natl Lab, Argonne, IL 60439 USA
[4] Shanghai Univ, Sch Environm & Chem Engn, Shanghai 200444, Peoples R China
关键词
VOLATILE ORGANIC-COMPOUNDS; CARBON EMISSIONS; BLACK CARBON; NOX; GASES; ASIA; SO2; SHANGHAI; HANGZHOU; AEROSOLS;
D O I
10.5194/acp-11-4105-2011
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
The purpose of this study is to develop an emission inventory for major anthropogenic air pollutants and VOC species in the Yangtze River Delta (YRD) region for the year 2007. A "bottom-up" methodology was adopted to compile the inventory based on major emission sources in the sixteen cities of this region. Results show that the emissions of SO2, NOx, CO, PM10, PM2.5, VOCs, and NH3 in the YRD region for the year 2007 are 2392 kt, 2293 kt, 6697 kt, 3116 kt, 1511 kt, 2767 kt, and 459 kt, respectively. Ethylene, mp-xylene, o-xylene, toluene, 1,2,4-trimethylbenzene, 2,4-dimethylpentane, ethyl benzene, propylene, 1-pentene, and isoprene are the key species contributing 77% to the total ozone formation potential (OFP). The spatial distribution of the emissions shows the emissions and OFPs are mainly concentrated in the urban and industrial areas along the Yangtze River and around Hangzhou Bay. The industrial sources, including power plants other fuel combustion facilities, and non-combustion processes contribute about 97%, 86%, 89%, 91%, and 69% of the total SO2, NOx, PM10, PM2.5, and VOC emissions. Vehicles take up 12.3% and 12.4% of the NOx and VOC emissions, respectively. Regarding OFPs, the chemical industry, domestic use of paint & printing, and gasoline vehicles contribute 38%, 24%, and 12% to the ozone formation in the YRD region.
引用
收藏
页码:4105 / 4120
页数:16
相关论文
共 61 条
[1]   DISTRIBUTION OF SO2, NOX AND CO2 EMISSIONS FROM FUEL COMBUSTION AND INDUSTRIAL ACTIVITIES IN ASIA WITH 1-DEGREES-X1-DEGREES RESOLUTION [J].
AKIMOTO, H ;
NARITA, H .
ATMOSPHERIC ENVIRONMENT, 1994, 28 (02) :213-225
[2]  
Amann M., 2008, Scenarios for Cost-Effective Control of Air Pollution and Greenhouse Gases in China.
[3]   Emission of trace gases and aerosols from biomass burning [J].
Andreae, MO ;
Merlet, P .
GLOBAL BIOGEOCHEMICAL CYCLES, 2001, 15 (04) :955-966
[4]  
[Anonymous], CHIN EN STAT YB 2008
[5]  
[Anonymous], AP42 USEPA
[6]  
[Anonymous], 2006, EMEP CORINAIR EM INV
[7]  
[Anonymous], CHIN STAT YB 2008
[8]   Spatial and temporal variation of historical anthropogenic NMVOCs emission inventories in China [J].
Bo, Y. ;
Cai, H. ;
Xie, S. D. .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2008, 8 (23) :7297-7316
[9]  
[曹国良 Cao Guoliang], 2005, [中国环境科学, China Environmental Science], V25, P389
[10]   Inventory of black carbon and organic carbon emissions from China [J].
Cao, Guoliang ;
Zhang, Xiaoye ;
Zheng, Fangcheng .
ATMOSPHERIC ENVIRONMENT, 2006, 40 (34) :6516-6527