Semiclassical description of photoionization microscopy -: art. no. 012709

被引:51
作者
Bordas, C
Lépine, F
Nicole, C
Vrakking, MJJ
机构
[1] CNRS, Spectrometrie Ion & Mol Lab, UMR 5579, F-69622 Villeurbanne, France
[2] FOM, Inst Atom & Mol Phys, NL-1098 SJ Amsterdam, Netherlands
来源
PHYSICAL REVIEW A | 2003年 / 68卷 / 01期
关键词
D O I
10.1103/PhysRevA.68.012709
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
Recently, experiments have been reported where a geometrical interference pattern was observed when photoelectrons ejected in the threshold photoionization of xenon were detected in a velocity-map imaging apparatus [C. Nicole , Phys. Rev. Lett. 88, 133001 (2002)]. This technique, called photoionization microscopy, relies on the existence of interferences between various trajectories by which the electron moves from the atom to the plane of observation. Unlike previous predictions relevant to the hydrogenic case, the structure of the interference pattern evolves smoothly with the excess energy above the saddle point and is only weakly affected by the presence of continuum Stark resonances. In this paper, we describe a semiclassical analysis of this process and present numerical simulations in excellent agreement with the experimental results. It is shown that the background contribution dominates in the observations, as opposed to the behavior expected for hydrogenic systems where the interference pattern is qualitatively different on quasidiscrete Stark resonances.
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页数:13
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