First-passage time of cyclization dynamics of a wormlike polymer

被引:17
作者
Chen, JZY [1 ]
Tsao, HK
Sheng, YJ
机构
[1] Univ Waterloo, Dept Phys, Waterloo, ON N2L 3G1, Canada
[2] Natl Cent Univ, Dept Chem & Mat Engn, Chungli 320, Taiwan
[3] Natl Taiwan Univ, Dept Chem Engn, Taipei 106, Taiwan
来源
EUROPHYSICS LETTERS | 2004年 / 65卷 / 03期
关键词
D O I
10.1209/epl/i2003-10086-2
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
The mean first-passage time of cyclization is investigated for a wormlike polymer chain with reactive ends. Using Monte Carlo simulations we examine the dependence of the mean first-passage time on the total number of monomers N and binding force range. We show that the mean first-passage time exhibits a minimum as N varies and display an exponentially large increase as the chain becomes stiff.
引用
收藏
页码:407 / 413
页数:7
相关论文
共 20 条
[1]  
BINDER K, 1988, MONTE CARLO SIMULATI, P45305
[2]  
DEGENNES PG, 1993, SCALING CONCEPTS POL, P45305
[3]  
DOI M, 1975, CHEM PHYS, V9, P455, DOI 10.1016/0301-0104(75)80083-8
[4]  
DOI M, 1988, THEORY POLYM DYNAMIC, P45305
[5]   The dynamics of chain closure in semiflexible polymers [J].
Dua, A ;
Cherayil, BJ .
JOURNAL OF CHEMICAL PHYSICS, 2002, 116 (01) :399-409
[6]   Dynamic fluctuations of semiflexible filaments [J].
Everaers, R ;
Jülicher, F ;
Ajdari, A ;
Maggs, AC .
PHYSICAL REVIEW LETTERS, 1999, 82 (18) :3717-3720
[7]   THEORY OF INTRAMOLECULAR REACTIONS IN POLYMERIC LIQUIDS [J].
FRIEDMAN, B ;
OSHAUGHNESSY, B .
MACROMOLECULES, 1993, 26 (18) :4888-4898
[8]   THEORY OF POLYMER CYCLIZATION [J].
FRIEDMAN, B ;
OSHAUGHNESSY, B .
PHYSICAL REVIEW A, 1989, 40 (10) :5950-5959
[9]   Diffusion-limited loop formation of semiflexible polymers: Kramers theory and the intertwined time scales of chain relaxation and closing [J].
Jun, S ;
Bechhoefer, J ;
Ha, BY .
EUROPHYSICS LETTERS, 2003, 64 (03) :420-426
[10]   Looping dynamics of linear DNA molecules and the effect of DNA curvature: A study by Brownian dynamics simulation [J].
Merlitz, H ;
Rippe, K ;
Klenin, KV ;
Langowski, J .
BIOPHYSICAL JOURNAL, 1998, 74 (02) :773-779