Pore-scale flow and mass transport in gas diffusion layer of proton exchange membrane fuel cell with interdigitated flow fields

被引:195
作者
Chen, Li [1 ]
Luan, Hui-Bao [1 ]
He, Ya-Ling [1 ]
Tao, Wen-Quan [1 ]
机构
[1] Xi An Jiao Tong Univ, Key Lab Thermal Fluid Sci & Engn MOE, Sch Energy & Power Engn, Xian 710049, Shaanxi, Peoples R China
基金
中国国家自然科学基金;
关键词
Proton exchange membrane fuel cell; Interdigitated flow field; Lattice Boltzmann method; Pore-scale; Mass transport; Liquid water; LATTICE BOLTZMANN METHOD; BOUNDARY-CONDITIONS; MATHEMATICAL-MODEL; WATER TRANSPORT; SIMULATION; PERFORMANCE; ELECTRODES; PRESSURE; CATHODE; PERMEABILITY;
D O I
10.1016/j.ijthermalsci.2011.08.003
中图分类号
O414.1 [热力学];
学科分类号
070201 [理论物理];
摘要
Lattice Boltzmann method (LBM) is employed to investigate pore-scale flow and mass transport in a carbon paper gas diffusion layer (GDL) of interdigitated PEMFC. The carbon paper GDL is reconstructed using the stochastic method, and its macroscopic transport properties are numerically predicted. The predicted anisotropic permeabilities and effective diffusivity of the reconstructed GDL agree well with existing measurements. Then, effects of the porous structures of the carbon paper GDL are explored in terms of fluid flow, species transport and electrochemical reaction. The GDL porous structures greatly affect flow and mass transport, creating distinct specie concentration distribution and local current density distribution. Besides, simulations are performed to explore liquid water behaviors in the reconstructed GDL The simulation results present a detailed description of the pore-scale liquid water behaviors. Further, simulations are performed to investigate the effects of land width and GDL contact angle on liquid water removal time and residual saturation. Narrower land reduces liquid water removal time and residual saturation. Higher contact angle increases the removal time and reduces the residual saturation. Crown Copyright (C) 2011 Published by Elsevier Masson SAS. All rights reserved.
引用
收藏
页码:132 / 144
页数:13
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