Ethane conversion in the presence of iron- and manganese-promoted sulfated zirconium dioxide: Evidence of autocatalysis and oligocondensation chemistry

被引:14
作者
Cheung, TK [1 ]
Gates, BC [1 ]
机构
[1] UNIV CALIF DAVIS,DEPT MAT SCI & CHEM ENGN,DAVIS,CA 95616
关键词
D O I
10.1039/cc9960001937
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Ethane reacts in the presence of Fe- and Mn-promoted sulfated ZrO2 to form butane, ethene, methane and H-2 at temperatures greater than or equal to 473 K; the data indicate autocatalysis with carbocation intermediates as in superacid solution chemistry.
引用
收藏
页码:1937 / 1938
页数:2
相关论文
共 9 条
  • [1] ISOMERIZATION OF C-13 LABELED BUTANE OVER FE,MN PROMOTED SULFATED ZRO2 CATALYST
    ADEEVA, V
    LEI, GD
    SACHTLER, WMH
    [J]. APPLIED CATALYSIS A-GENERAL, 1994, 118 (01) : L11 - L15
  • [2] ACID SITES IN SULFATED AND METAL-PROMOTED ZIRCONIUM DIOXIDE CATALYSTS
    ADEEVA, V
    DEHAAN, JW
    JANCHEN, J
    LEI, GD
    SCHUNEMANN, V
    VANDEVEN, LJM
    SACHTLER, WMH
    VANSANTEN, RA
    [J]. JOURNAL OF CATALYSIS, 1995, 151 (02) : 364 - 372
  • [3] LOW-TEMPERATURE SUPERACID CATALYSIS - REACTIONS OF N-BUTANE CATALYZED BY IRON-PROMOTED AND MANGANESE-PROMOTED SULFATED ZIRCONIA
    CHEUNG, TK
    DITRI, JL
    GATES, BC
    [J]. JOURNAL OF CATALYSIS, 1995, 151 (02) : 464 - 466
  • [4] Propane conversion catalyzed by sulfated zirconia, iron- and manganese-promoted sulfated zirconia, and USY zeolite
    Cheung, TK
    Lange, FC
    Gates, BC
    [J]. JOURNAL OF CATALYSIS, 1996, 159 (01) : 99 - 106
  • [5] PROPANE CONVERSION IN THE PRESENCE OF IRON-PROMOTED AND MANGANESE-PROMOTED SULFATED ZIRCONIA - EVIDENCE OF OLAH CARBOCATION CHEMISTRY
    CHEUNG, TK
    LANGE, FC
    GATES, BC
    [J]. CATALYSIS LETTERS, 1995, 34 (3-4) : 351 - 358
  • [6] A HIGHLY-ACTIVE SOLID SUPERACID CATALYST FOR N-BUTANE ISOMERIZATION - A SULFATED OXIDE CONTAINING IRON, MANGANESE AND ZIRCONIUM
    HSU, CY
    HEIMBUCH, CR
    ARMES, CT
    GATES, BC
    [J]. JOURNAL OF THE CHEMICAL SOCIETY-CHEMICAL COMMUNICATIONS, 1992, (22) : 1645 - 1646
  • [7] DETECTION OF SUPERACIDITY ON SOLID SUPERACIDS - A NEW APPROACH
    LIN, CH
    HSU, CY
    [J]. JOURNAL OF THE CHEMICAL SOCIETY-CHEMICAL COMMUNICATIONS, 1992, (20) : 1479 - 1480
  • [8] ELECTROPHILIC REACTIONS AT SINGLE BONDS .12. HYDROGEN-DEUTERIUM EXCHANGE, PROTOLYSIS (DEUTEROLYSIS), AND OLIGOCONDENSATION OF ALKANES WITH SUPERACIDS
    OLAH, GA
    HALPERN, Y
    SHEN, J
    MO, YK
    [J]. JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 1973, 95 (15) : 4960 - 4970
  • [9] STRUCTURE OF FE, MN-PROMOTED SULFATED ZIRCONIA CATALYST BY X-RAY AND IN ABSORPTION SPECTROSCOPIES
    TABORA, JE
    DAVIS, RJ
    [J]. JOURNAL OF THE CHEMICAL SOCIETY-FARADAY TRANSACTIONS, 1995, 91 (12): : 1825 - 1833