Characterization of nanometer-sized, mechanically exfoliated graphene on the H-passivated Si(100) surface using scanning tunneling microscopy

被引:55
作者
Ritter, Kyle A. [1 ,2 ]
Lyding, Joseph W. [1 ,3 ]
机构
[1] Univ Illinois, Beckman Inst Adv Sci & Technol, Urbana, IL 61801 USA
[2] Univ Illinois, Dept Mat Sci & Engn, Urbana, IL 61801 USA
[3] Univ Illinois, Dept Elect & Comp Engn, Urbana, IL 61801 USA
关键词
D O I
10.1088/0957-4484/19/01/015704
中图分类号
TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
We have developed a method for depositing graphene monolayers and bilayers with minimum lateral dimensions of 2-10 nm by the mechanical exfoliation of graphite onto the Si(100)-2 x 1:H surface. Room temperature, ultrahigh vacuum tunneling spectroscopy measurements of nanometer-sized single layer graphene reveal a size-dependent energy gap ranging from 0.1 to 1 eV. Furthermore, the number of graphene layers can be directly determined from scanning tunneling microscopy topographic contours. This atomistic study provides an experimental basis for probing the electronic structure of nanometer-sized graphene which can assist the development of graphene-based nanoelectronics.
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页数:6
相关论文
共 33 条
[1]   Scanning tunnelling spectroscopy and ab initio calculations of single-walled carbon nanotubes interfaced with highly doped hydrogen-passivated Si(100) substrates [J].
Albrecht, Peter M. ;
Barraza-Lopez, Salvador ;
Lyding, Joseph W. .
NANOTECHNOLOGY, 2007, 18 (09)
[2]   Preferential orientation of a chiral semiconducting carbon nanotube on the locally depassivated Si(100)-2x1:H surface identified by scanning Tunneling microscopy [J].
Albrecht, Peter M. ;
Barraza-Lopez, Salvador ;
Lyding, Joseph W. .
SMALL, 2007, 3 (08) :1402-1406
[3]  
Albrecht PM, 2007, NANOTECHNOLOGY, V18, DOI [10.1088/0957-4484/18/12/125302, 10.1088/0957/18/12/125302]
[4]  
Albrecht PM, 2004, AIP CONF PROC, V723, P173, DOI 10.1063/1.1812067
[5]   Ultrahigh-vacuum scanning tunneling microscopy and spectroscopy of single-walled carbon nanotubes on hydrogen-passivated Si(100) surfaces [J].
Albrecht, PM ;
Lyding, JW .
APPLIED PHYSICS LETTERS, 2003, 83 (24) :5029-5031
[6]  
[Anonymous], 1993, INTRO SCANNING TUNNE
[7]  
ARESHKIN DA, 2007, NANO LETT, DOI DOI 10.1021/NL07078C
[8]   Electronic structure and stability of semiconducting graphene nanoribbons [J].
Barone, Veronica ;
Hod, Oded ;
Scuseria, Gustavo E. .
NANO LETTERS, 2006, 6 (12) :2748-2754
[9]   Ultrathin epitaxial graphite: 2D electron gas properties and a route toward graphene-based nanoelectronics [J].
Berger, C ;
Song, ZM ;
Li, TB ;
Li, XB ;
Ogbazghi, AY ;
Feng, R ;
Dai, ZT ;
Marchenkov, AN ;
Conrad, EH ;
First, PN ;
de Heer, WA .
JOURNAL OF PHYSICAL CHEMISTRY B, 2004, 108 (52) :19912-19916
[10]   Scanning tunneling spectroscopy of inhomogeneous electronic structure in monolayer and bilayer graphene on SiC [J].
Brar, Victor W. ;
Zhang, Yuanbo ;
Yayon, Yossi ;
Ohta, Taisuke ;
McChesney, Jessica L. ;
Bostwick, Aaron ;
Rotenberg, Eli ;
Horn, Karsten ;
Crommie, Michael F. .
APPLIED PHYSICS LETTERS, 2007, 91 (12)