Scintillation properties of LuI3:Ce3+-high light yield scintillators

被引:44
作者
Birowosuto, MD
Dorenbos, P
van Eijk, CWE
Krämer, KW
Güdel, HU
机构
[1] Delft Univ Technol, Inst Interfac Reactor, Radiat Technol Grp, NL-2629 JB Delft, Netherlands
[2] Univ Bern, Dept Chem & Biochem, CH-3000 Bern, Switzerland
关键词
Ce3+; decay time; lanthanide trihalide; light yield; LuI3; nonproportionality; scintillator;
D O I
10.1109/TNS.2005.852630
中图分类号
TM [电工技术]; TN [电子技术、通信技术];
学科分类号
0808 ; 0809 ;
摘要
The scintillation properties of LuI3:Ce3+ (Pure, 0.5%,. 2%, and 5% Ce3+), a new member of the generation of Ce3+ doped lanthanide trihalide scintillators, are presented. This material has a calculated density of 5.6 g/cm(3) and an atomic number Z(eff) of 60.2. Under optical and X-ray excitation, Ce3+ emission is observed to peak at 472 and 535 nm. A high light yield of 76000 photons per MeV (ph/MeV) was measured for LuI3:2% Ce3+. LuI3:Ce3+ has a nonexponential decay time. The contribution of short decay components (within 50 ns) to the total light yield is around 50%. An energy resolution (full-width half maximum over peak position) for the 662 keV full energy peak of 4.7 +/- 0.5% was observed for LU13:0-5% Ce3+.
引用
收藏
页码:1114 / 1118
页数:5
相关论文
共 14 条
[1]   PREPARATION + CRYSTAL DATA FOR LANTHANIDE + ACTINIDE TRIIODIDES [J].
ASPREY, LB ;
KRUSE, FH ;
KEENAN, TK .
INORGANIC CHEMISTRY, 1964, 3 (08) :1137-&
[2]  
ASTAKHOVA IS, 1992, R J INORG CHEM, V37, P1376
[3]   Luminescence and scintillation properties of the small band gap compound LaI3:Ce3+ [J].
Bessiere, A ;
Dorenbos, P ;
van Eijk, CWE ;
Krämer, KW ;
Güdel, HU ;
Donega, CD ;
Meijerink, A .
NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT, 2005, 537 (1-2) :22-26
[4]   MEASUREMENT OF TIME DEPENDENCE OF SCINTILLATION INTENSITY BY A DELAYED-COINCIDENCE METHOD [J].
BOLLINGER, L ;
THOMAS, GE .
REVIEW OF SCIENTIFIC INSTRUMENTS, 1961, 32 (09) :1044-+
[5]   Measuring the absolute light yield of scintillators [J].
de Haas, JTM ;
Dorenbos, P ;
van Eijk, CWE .
NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT, 2005, 537 (1-2) :97-100
[6]  
DORENBOS P, 2003, P KEK NCRP INT SCH M, P15
[7]  
GLODO J, UNPUB NUCL INSTRUM A
[8]   Optical and scintillation properties of cerium-doped LaCl3, LuBr3 and LuCl3 [J].
Guillot-Noël, O ;
de Haas, JTM ;
Dorenbos, P ;
van Eijk, CWE ;
Krämer, K ;
Güdel, HU .
JOURNAL OF LUMINESCENCE, 1999, 85 (1-3) :21-35
[9]   A METHOD TO INCREASE OPTICAL TIMING SPECTRA MEASUREMENT RATES USING A MULTI-HIT TDC [J].
MOSES, WW .
NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT, 1993, 336 (1-2) :253-261
[10]   LuI3: Ce - A new scintillator for gamma ray spectroscopy [J].
Shah, KS ;
Glodo, J ;
Klugerman, M ;
Higgins, W ;
Gupta, T ;
Wong, P ;
Moses, WW ;
Derenzo, SE ;
Weber, MJ ;
Dorenbos, P .
IEEE TRANSACTIONS ON NUCLEAR SCIENCE, 2004, 51 (05) :2302-2305