Assessing future nitrogen deposition and carbon cycle feedback using a multimodel approach: Analysis of nitrogen deposition

被引:249
作者
Lamarque, JF [1 ]
Kiehl, JT
Brasseur, GP
Butler, T
Cameron-Smith, P
Collins, WD
Collins, WJ
Granier, C
Hauglustaine, D
Hess, PG
Holland, EA
Horowitz, L
Lawrence, MG
McKenna, D
Merilees, P
Prather, MJ
Rasch, PJ
Rotman, D
Shindell, D
Thornton, P
机构
[1] Natl Ctr Atmospher Res, Boulder, CO 80305 USA
[2] Max Planck Inst Meteorol, D-20146 Hamburg, Germany
[3] Max Planck Inst Chem, D-55128 Mainz, Germany
[4] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA
[5] Met Off, Hadley Ctr, Exeter EX1 3PB, Devon, England
[6] Inst Pierre Simon Laplace, Serv Aeron, Paris, France
[7] NOAA, CIRES, Aeron Lab, Boulder, CO USA
[8] Inst Pierre Simon Laplace, Lab Sci Climat & Environm, F-91191 Gif Sur Yvette, France
[9] NOAA, Geophys Fluid Dynam Lab, Princeton, NJ 08542 USA
[10] Univ Calif Irvine, Irvine, CA 92697 USA
[11] NASA, Goddard Inst Space Studies, New York, NY 10025 USA
关键词
D O I
10.1029/2005JD005825
中图分类号
P4 [大气科学(气象学)];
学科分类号
0706 ; 070601 ;
摘要
[1] In this study, we present the results of nitrogen deposition on land from a set of 29 simulations from six different tropospheric chemistry models pertaining to present-day and 2100 conditions. Nitrogen deposition refers here to the deposition ( wet and dry) of all nitrogen-containing gas phase chemical species resulting from NOx (NO + NO2) emissions. We show that under the assumed IPCC SRES A2 scenario the global annual average nitrogen deposition over land is expected to increase by a factor of similar to 2.5, mostly because of the increase in nitrogen emissions. This will significantly expand the areas with annual average deposition exceeding 1 gN/m(2)/year. Using the results from all models, we have documented the strong linear relationship between models on the fraction of the nitrogen emissions that is deposited, regardless of the emissions ( present day or 2100). On average, approximately 70% of the emitted nitrogen is deposited over the landmasses. For present-day conditions the results from this study suggest that the deposition over land ranges between 25 and 40 Tg(N)/year. By 2100, under the A2 scenario, the deposition over the continents is expected to range between 60 and 100 Tg( N)/year. Over forests the deposition is expected to increase from 10 Tg( N)/year to 20 Tg( N)/year. In 2100 the nitrogen deposition changes from changes in the climate account for much less than the changes from increased nitrogen emissions.
引用
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页码:1 / 21
页数:21
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