We report the first observation of photon antibunching in the photoluminescence from single carbon nanotubes. The emergence of a fast luminescence decay component under strong optical excitation indicates that Auger processes are partially responsible for inhibiting two-photon generation. Additionally, the presence of exciton localization at low temperatures ensures that nanotubes emit photons predominantly one by one. The fact that multiphoton emission probability can be smaller than 5% suggests that carbon nanotubes could be used as a source of single photons for applications in quantum cryptography.
机构:
Max Planck Gesell, Fritz Haber Inst, Dept Phys Chem, D-12489 Berlin, GermanyMax Planck Gesell, Fritz Haber Inst, Dept Phys Chem, D-12489 Berlin, Germany
Hagen, A
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Steiner, M
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机构:Max Planck Gesell, Fritz Haber Inst, Dept Phys Chem, D-12489 Berlin, Germany
Steiner, M
;
Raschke, MB
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机构:Max Planck Gesell, Fritz Haber Inst, Dept Phys Chem, D-12489 Berlin, Germany
Raschke, MB
;
Lienau, C
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机构:Max Planck Gesell, Fritz Haber Inst, Dept Phys Chem, D-12489 Berlin, Germany
Lienau, C
;
Hertel, T
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机构:Max Planck Gesell, Fritz Haber Inst, Dept Phys Chem, D-12489 Berlin, Germany
Hertel, T
;
Qian, HH
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机构:Max Planck Gesell, Fritz Haber Inst, Dept Phys Chem, D-12489 Berlin, Germany
Qian, HH
;
Meixner, AJ
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机构:Max Planck Gesell, Fritz Haber Inst, Dept Phys Chem, D-12489 Berlin, Germany
Meixner, AJ
;
Hartschuh, A
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机构:Max Planck Gesell, Fritz Haber Inst, Dept Phys Chem, D-12489 Berlin, Germany
机构:
Max Planck Gesell, Fritz Haber Inst, Dept Phys Chem, D-12489 Berlin, GermanyMax Planck Gesell, Fritz Haber Inst, Dept Phys Chem, D-12489 Berlin, Germany
Hagen, A
;
Steiner, M
论文数: 0引用数: 0
h-index: 0
机构:Max Planck Gesell, Fritz Haber Inst, Dept Phys Chem, D-12489 Berlin, Germany
Steiner, M
;
Raschke, MB
论文数: 0引用数: 0
h-index: 0
机构:Max Planck Gesell, Fritz Haber Inst, Dept Phys Chem, D-12489 Berlin, Germany
Raschke, MB
;
Lienau, C
论文数: 0引用数: 0
h-index: 0
机构:Max Planck Gesell, Fritz Haber Inst, Dept Phys Chem, D-12489 Berlin, Germany
Lienau, C
;
Hertel, T
论文数: 0引用数: 0
h-index: 0
机构:Max Planck Gesell, Fritz Haber Inst, Dept Phys Chem, D-12489 Berlin, Germany
Hertel, T
;
Qian, HH
论文数: 0引用数: 0
h-index: 0
机构:Max Planck Gesell, Fritz Haber Inst, Dept Phys Chem, D-12489 Berlin, Germany
Qian, HH
;
Meixner, AJ
论文数: 0引用数: 0
h-index: 0
机构:Max Planck Gesell, Fritz Haber Inst, Dept Phys Chem, D-12489 Berlin, Germany
Meixner, AJ
;
Hartschuh, A
论文数: 0引用数: 0
h-index: 0
机构:Max Planck Gesell, Fritz Haber Inst, Dept Phys Chem, D-12489 Berlin, Germany