Charged particle tracks in water of different phases. Monte Carlo simulation of electron tracks

被引:32
作者
Bigildeev, EA [1 ]
Michalik, V [1 ]
机构
[1] INST PHYS NUCL,DEPT RADIAT DOSIMETRY,CR-18086 PRAGUE 8,CZECH REPUBLIC
关键词
D O I
10.1016/0969-806X(95)00002-F
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The paper describes the energy deposition by charged particles in gaseous and liquid water. Cross sections and other important quantities as integral W-values, initial yields of ionizations and excitations, slowing down spectra etc. are reported and compared with available data. Track structure calculations for low energy electrons have been performed using Monte Carlo models. The frequency distributions of numbers of ionizations and excitations produced in water vapor and liquid water have been calculated. The spatial distribution of initial radiation products in electron tracks produced in both phases are also compared. The point-pair distributions of distances between the following pairs were studied: ionization-ionization, ionization-excitation, excitation-excitation and between all inelastic events (ionizations and excitations). The results obtained show significant physical differences between both phases which can lead to considerable differences in stochastic chemistry calculations.
引用
收藏
页码:197 / 207
页数:11
相关论文
共 41 条
  • [1] X-RAY PHOTOELECTRON-SPECTROSCOPY OF AMORPHOUS ICE
    BARON, B
    WILLIAMS, F
    [J]. JOURNAL OF CHEMICAL PHYSICS, 1976, 64 (09) : 3896 - 3897
  • [2] BEDNAR J, 1991, THEORETICAL F RAD CH
  • [3] BRENNER DJ, 1988, RADIAT PHYS CHEM, V32, P157
  • [4] Brenner DJ, 1983, PHYS MED BIOL, V29, P443
  • [5] CHRISTOPHOROU LG, 1971, ATOMIC MOL RAD PHYSI, pCH2
  • [6] MEASUREMENT OF W-VALUES OF LOW-ENERGY ELECTRONS IN SEVERAL GASES
    COMBECHER, D
    [J]. RADIATION RESEARCH, 1980, 84 (02) : 189 - 218
  • [7] GREEN NJB, 1988, RADIAT PHYS CHEM, V32, P99
  • [8] TRANSPORT OF LOW-ENERGY ELECTRONS IN NITROGEN AND AIR
    GROSSWENDT, B
    WAIBEL, E
    [J]. NUCLEAR INSTRUMENTS & METHODS, 1978, 155 (1-2): : 145 - 156
  • [9] CALCULATION OF HEAVY-ION TRACKS IN LIQUID WATER
    HAMM, RN
    TURNER, JE
    RITCHIE, RH
    WRIGHT, HA
    [J]. RADIATION RESEARCH, 1985, 104 (02) : S20 - S26
  • [10] COLLECTIVE OSCILLATION IN LIQUID WATER
    HELLER, JM
    HAMM, RN
    BIRKHOFF, RD
    PAINTER, LR
    [J]. JOURNAL OF CHEMICAL PHYSICS, 1974, 60 (09) : 3483 - 3486