Evidence for an unconventional magnetic instability in the spin-tetrahedra system Cu2Te2O5Br2 -: art. no. 227201

被引:74
作者
Lemmens, P [1 ]
Choi, KY
Kaul, EE
Geibel, C
Becker, K
Brenig, W
Valenti, R
Gros, C
Johnsson, M
Millet, P
Mila, F
机构
[1] Rhein Westfal TH Aachen, Inst Phys 2, D-56056 Aachen, Germany
[2] Max Planck Inst Chem Phys Stoffe, D-01187 Dresden, Germany
[3] Tech Univ Dresden, Inst Theoret Phys, D-01069 Dresden, Germany
[4] Univ Saarland, Inst Theoret Phys, D-66041 Saarbrucken, Germany
[5] Univ Stockholm, Dept Inorgan Chem, S-10691 Stockholm, Sweden
[6] CNRS, Ctr Elaborat Mat & Etud Struct, F-31062 Toulouse, France
[7] Univ Lausanne, Inst Phys Theor, CH-1015 Lausanne, Switzerland
[8] Tech Univ Braunschweig, Inst Theoret Phys, D-3300 Braunschweig, Germany
关键词
D O I
10.1103/PhysRevLett.87.227201
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
Thermodynamic experiments as well as Raman scattering have been used to study the magnetic instabilities in the spin-tetrahedra systems Cu2Te2O5X2, X = Cl and Br. While the phase transition observed in the Cl system at T-N = 18.2 K is consistent with 3D antiferromagnetic ordering, the phase transition at T-o = 11.4 K in the Br system has several unusual features. We propose an explanation in terms of weakly coupled tetrahedra with a singlet-triplet gap and low-lying singlets.
引用
收藏
页码:227201 / 227201
页数:4
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