Stratospheric mean ages and transport rates from observations of carbon dioxide and nitrous oxide

被引:176
作者
Boering, KA
Wofsy, SC
Daube, BC
Schneider, HR
Loewenstein, M
Podolske, JR
机构
[1] HARVARD UNIV,DIV ENGN & APPL SCI,CAMBRIDGE,MA 02138
[2] HARVARD UNIV,DEPT EARTH & PLANETARY SCI,CAMBRIDGE,MA 02138
[3] NASA,AMES RES CTR,MOFFETT FIELD,CA 94035
[4] NOAA,CLIMATE MONITORING & DIAGNOST LAB,BOULDER,CO 80303
关键词
D O I
10.1126/science.274.5291.1340
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
Measurements of stratospheric carbon dioxide (CO2) and nitrous oxide (N2O) concentrations were analyzed to investigate stratospheric transport rates. Temporal variations in tropospheric CO2 were observed to propagate into the stratosphere, showing that tropospheric air enters the lower tropical stratosphere continuously, ascends, and is transported rapidly (in less than 1 month) to both hemispheres. The mean age A of stratospheric air determined from CO2 data is approximately 5 years in the mid-stratosphere. The mean age is mathematically equivalent to a conserved tracer analogous to exhaust from stratospheric aircraft. Comparison of values for A from models and observations indicates that current model simulations likely underestimate pollutant concentrations from proposed stratospheric aircraft by 25 to 100 percent.
引用
收藏
页码:1340 / 1343
页数:4
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