Chemical reduction of CO2 to different products during photo catalytic reaction on TiO2 under diverse conditions:: an overview

被引:201
作者
Dey, G. R. [1 ]
机构
[1] Bhabha Atom Res Ctr, Radiat & Photochem Div, Bombay 400085, Maharashtra, India
来源
JOURNAL OF NATURAL GAS CHEMISTRY | 2007年 / 16卷 / 03期
关键词
CO2 chemical reduction; H-2; CH4; CO; TiO2; hole scavenger; photolysis;
D O I
10.1016/S1003-9953(07)60052-8
中图分类号
O69 [应用化学];
学科分类号
081704 [应用化学];
摘要
The chemical reduction of CO2 remains a challenge with respect to the reversal of the oxidative degradation of any organic materials. The conversion of CO2 into useful substances is essential in developing alternative fuels and various raw materials for different industries. This also aids in preventing the continuous rise in tropospheric temperature due to the green house effect of CO2. In this article an overview of the growth taken place so far in the field of CO2 chemical reduction is presented. The discussion comprises of photochemical methods for the development of different products, viz. CO, CH3OH and CH4, through chemical reduction of CO2. This includes the use of photo catalysts, mainly TiO2, and the role of a hole scavenger (such as 2-propanol) for this purpose.
引用
收藏
页码:217 / 226
页数:10
相关论文
共 76 条
[1]
PHOTOCATALYTIC DEHYDROGENATION OF ISOPROPANOL ON PT/TIO2 CATALYSTS [J].
AITICHOU, I ;
FORMENTI, M ;
POMMIER, B ;
TEICHNER, SJ .
JOURNAL OF CATALYSIS, 1985, 91 (02) :293-307
[3]
PHOTOCATALYTIC REDUCTION OF CO2 WITH H2O ON VARIOUS TITANIUM-OXIDE CATALYSTS [J].
ANPO, M ;
YAMASHITA, H ;
ICHIHASHI, Y ;
EHARA, S .
JOURNAL OF ELECTROANALYTICAL CHEMISTRY, 1995, 396 (1-2) :21-26
[4]
BAHNEMANN DW, 1991, PHOTOCHEMICAL CONVERSION AND STORAGE OF SOLAR ENERGY, P251
[5]
PHOTOADSORPTION AND PHOTOCATALYSIS AT RUTILE SURFACES .2. PHOTOCATALYTIC OXIDATION OF ISOPROPANOL [J].
BICKLEY, RI ;
MUNUERA, G ;
STONE, FS .
JOURNAL OF CATALYSIS, 1973, 31 (03) :398-407
[6]
PHOTO-ADSORPTION AND PHOTO-CATALYSIS ON TITANIUM-DIOXIDE SURFACES - PHOTO-ADSORPTION OF OXYGEN AND PHOTOCATALYZED OXIDATION OF ISOPROPANOL [J].
BICKLEY, RI ;
JAYANTY, RKM .
FARADAY DISCUSSIONS, 1974, 58 :194-204
[7]
Bieski B. H. J., 1985, J PHYS CHEM REF DATA, V14, P1041
[8]
Photocatalytic dehydrogenation of 2-propanol on TiO2(110) [J].
Brinkley, D ;
Engel, T .
JOURNAL OF PHYSICAL CHEMISTRY B, 1998, 102 (39) :7596-7605
[9]
CRITICAL-REVIEW OF RATE CONSTANTS FOR REACTIONS OF HYDRATED ELECTRONS, HYDROGEN-ATOMS AND HYDROXYL RADICALS (.OH/.O-) IN AQUEOUS-SOLUTION [J].
BUXTON, GV ;
GREENSTOCK, CL ;
HELMAN, WP ;
ROSS, AB .
JOURNAL OF PHYSICAL AND CHEMICAL REFERENCE DATA, 1988, 17 (02) :513-886
[10]
Chatwal G., 1985, SPECTROSCOPY ATOMIC, P110