Reentrant morphology transition in the growth of free silver nanoclusters

被引:130
作者
Baletto, F
Mottet, C
Ferrando, R
机构
[1] INFM, I-16146 Genoa, Italy
[2] Univ Genoa, Dipartimento Fis, CNR, CFSBT, I-16146 Genoa, Italy
[3] CNRS, CRMC2, F-13288 Marseille 9, France
关键词
D O I
10.1103/PhysRevLett.84.5544
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
The growth of free silver nanoclusters is studied by molecular dynamics simulations, from a small seed up to sizes N similar or equal to 150. It is Shown that the final outcome of the growth process depends crucially on the growth conditions (deposition flux phi and temperature T). A reentrant morphology transition is obtained: at intermediate values of T and phi a "decahedral window" is found; the window is surrounded by regimes where icosahedra are preferentially grown.
引用
收藏
页码:5544 / 5547
页数:4
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