Characterization of Silica Supported Nickel Catalyst for Methanation with Improved Activity by Room Temperature Plasma Treatment

被引:37
作者
Shi, Peng [1 ]
Liu, Chang-Jun [1 ]
机构
[1] Tianjin Univ, Key Lab Green Chem Technol, Minist Educ, Sch Chem Engn & Technol, Tianjin 300072, Peoples R China
基金
中国国家自然科学基金;
关键词
Ni/SiO2; Impregnation; Plasma; CO hydrogenation; NI/AL2O3; CATALYST; CARBON DEPOSITION; CO DISSOCIATION; REMOVAL; NI; PRETREATMENT; MONOXIDE; ALUMINA; STREAM; SIZE;
D O I
10.1007/s10562-009-0163-0
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Room temperature glow discharge plasma was applied to treat the nickel precursor supported on SiO2. According to the catalyst characterization, the calcination thermally of the plasma treated sample shows small particle size and high dispersion. Such prepared sample presents high conversions of carbon monoxide and hydrogen for the reaction of methanation with a significantly improved anti-carbon deposition performance. The plasma-treated sample shows enhanced metal-support interaction and keeps good dispersion after reaction.
引用
收藏
页码:112 / 118
页数:7
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