We present a spectroscopic analysis and laser characterization of optically written waveguides in neodymium-doped gallium lanthanum sulphide (Nd3+-Ga:La:S) chalcogenide glass. Uniform channel waveguides were fabricated in Nd3+-Ga:La-S by exposure to radiation from a focused UV-laser beam (gimel = 244 nm), producing a refractive index change Deltan approximate to +10(-3). The observed laser performance and fluorescence decay were in good agreement with values calculated from a spectroscopic analysis of 85 mus for the F-4(3/2) lifetime and 5.9 x 10(-20) cm(2) for the emission cross section at 1075 nm. Low threshold laser operation with emission at 1075 nm and a slope efficiency of 17% is demonstrated. The active device is spatially single mode and exhibits up to 8.6 mW of output power and propagation losses of < 0.5 dB cm(-1). Waveguide fabrication, photoinduced effects, and optical characterization in terms of spectroscopy, laser performance, and device attenuation are discussed.