Steam gasification of almond shells in a fluidised bed reactor: The influence of temperature and particle size on product yield and distribution

被引:99
作者
Rapagna, S
Latif, A
机构
[1] Dipartimento di Chimica, Ingegneria Chimica e Materiali, Università di L'Aquila
关键词
biomass; almond shells; fluidised bed; gasification; hydrogen;
D O I
10.1016/S0961-9534(96)00079-7
中图分类号
S2 [农业工程];
学科分类号
0828 ;
摘要
The steam gasification of ground almond shells has been carried out in a continuous, bench scale, fluidised bed reactor in order to evaluate the effects of particle size and operating temperature on the product yield and distribution. The mean particle size was varied from nearly 300 mu m to over 1 mm and the bed temperature from 600 to 800 degrees C. The results reveal that for smaller particle sizes differences in product yield and distribution practically disappear as the higher temperature bound is approached, whereas for particles above 1 mm in diameter the yield continues to increase over the entire temperature range, never reaching that attained by the smaller particle systems. This behaviour is indicative of the increasing significance of extra- and/or intra-particle heat transfer limitations with increasing particle size. (C) 1997 Elsevier Science Ltd.
引用
收藏
页码:281 / 288
页数:8
相关论文
共 16 条
[1]   STEAM GASIFICATION OF BIOMASS WITH NICKEL SECONDARY CATALYSTS [J].
BAKER, EG ;
MUDGE, LK ;
BROWN, MD .
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 1987, 26 (07) :1335-1339
[2]   INFLUENCE OF PHYSICAL AND CHEMICAL-PARAMETERS ON WOOD PYROLYSIS [J].
BEAUMONT, O ;
SCHWOB, Y .
INDUSTRIAL & ENGINEERING CHEMISTRY PROCESS DESIGN AND DEVELOPMENT, 1984, 23 (04) :637-641
[3]   STEAM GASIFICATION OF CELLULOSIC WASTES IN A FLUIDIZED-BED WITH DOWNSTREAM VESSELS [J].
CORELLA, J ;
AZNAR, MP ;
DELGADO, J ;
ALDEA, E .
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 1991, 30 (10) :2252-2262
[4]  
Dalla Valle J. M., 1948, MICROMERITICS
[5]   Kinetic and heat transfer control in the slow and flash pyrolysis of solids [J].
DiBlasi, C .
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 1996, 35 (01) :37-46
[6]   Influences of model assumptions on the predictions of cellulose pyrolysis in the heat transfer controlled regime [J].
DiBlasi, C .
FUEL, 1996, 75 (01) :58-66
[7]  
DURAISWAMI K, 1991, AM CHEM SOC DIV FUEL, V36, P1677
[8]  
ERGUN S, 1952, CHEM ENG PROG, V48, P89
[9]   STEAM GASIFICATION OF LIGNOCELLULOSIC RESIDUES IN A FLUIDIZED-BED AT A SMALL PILOT SCALE - EFFECT OF THE TYPE OF FEEDSTOCK [J].
HERGUIDO, J ;
CORELLA, J ;
GONZALEZSAIZ, J .
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 1992, 31 (05) :1274-1282
[10]   MODELING OF THE PYROLYSIS OF BIOMASS PARTICLES - STUDIES ON KINETICS, THERMAL AND HEAT-TRANSFER EFFECTS [J].
KOUFOPANOS, CA ;
PAPAYANNAKOS, N ;
MASCHIO, G ;
LUCCHESI, A .
CANADIAN JOURNAL OF CHEMICAL ENGINEERING, 1991, 69 (04) :907-915