An experimental study on the effect of ultrasonication on viscosity and heat transfer performance of multi-wall carbon nanotube-based aqueous nanofluids

被引:432
作者
Garg, Paritosh [2 ]
Alvarado, Jorge L. [1 ]
Marsh, Charles [3 ,4 ]
Carlson, Thomas A. [3 ]
Kessler, David A. [5 ]
Annamalai, Kalyan [2 ]
机构
[1] Texas A&M Univ, Dept Engn Technol & Ind Distribut, College Stn, TX 77843 USA
[2] Texas A&M Univ, Dept Mech Engn, College Stn, TX 77843 USA
[3] USA, Ctr Res Dev & Engn, Construct Engn Res Lab, Champaign, IL 61822 USA
[4] Dept Nucl Plasma & Radiol Engn, Urbana, IL 61801 USA
[5] USN, Res Lab, Computat Phys & Fluid Dynam Lab, Washington, DC 20375 USA
基金
美国国家科学基金会;
关键词
Convective heat transfer; Nanofluids; Multi-walled; Carbon nanotubes; Thermal conductivity; Viscosity; Heat transfer enhancement; Non-Newtonian fluid; TEM; THERMAL-CONDUCTIVITY ENHANCEMENT; LAMINAR-FLOW; SUSPENSIONS;
D O I
10.1016/j.ijheatmasstransfer.2009.04.029
中图分类号
O414.1 [热力学];
学科分类号
摘要
Four samples of 1 wt% multi-walled carbon nanotube-based (MWCNT) aqueous nanofluids prepared via ultrasonication were thermally characterized. Direct imaging was done using a newly developed wet-TEM technique to assess the dispersion state of carbon nanotubes (CNT) in suspension. The effect of dispersing energy (ultrasonication) on viscosity, thermal conductivity, and the laminar convective heat transfer was studied. Results indicate that thermal conductivity and heat transfer enhancement increased until an optimum ultrasonication time was reached, and decreased on further ultrasonication. The suspensions exhibited a shear thinning behavior, which followed the Power Law viscosity model. The maximum enhancements in thermal conductivity and convective heat transfer were found to be 20% and 32%, respectively. The thermal conductivity enhancement increased considerably at temperatures greater than 24 degrees C. The enhancement in convective heat transfer was found to increase with axial distance. A number of mechanisms related to boundary layer thickness, micro-convective effect, particle rearrangement, possible induced convective effects due to temperature and viscosity variations in the radial direction, and the non-Newtonian nature of the samples are discussed. (C) 2009 Elsevier Ltd. All rights reserved.
引用
收藏
页码:5090 / 5101
页数:12
相关论文
共 32 条
[1]   AUGMENTATION OF HEAT TRANSPORT IN LAMINAR-FLOW OF POLYSTYRENE SUSPENSIONS .2. ANALYSIS OF DATA [J].
AHUJA, AS .
JOURNAL OF APPLIED PHYSICS, 1975, 46 (08) :3417-3425
[2]  
Alloush A., 1982, International Journal of Thermophysics, V3, P225, DOI 10.1007/BF00503318
[3]   Thermal conductivity enhancement in aqueous suspensions of carbon multi-walled and double-walled nanotubes in the presence of two different dispersants [J].
Assael, MJ ;
Metaxa, IN ;
Arvanitidis, J ;
Christofilos, D ;
Lioutas, C .
INTERNATIONAL JOURNAL OF THERMOPHYSICS, 2005, 26 (03) :647-664
[4]   Thermal conductivity of suspensions of carbon nanotubes in water [J].
Assael, MJ ;
Chen, CF ;
Metaxa, I ;
Wakeham, WA .
INTERNATIONAL JOURNAL OF THERMOPHYSICS, 2004, 25 (04) :971-985
[5]   Stabilization of individual carbon nanotubes in aqueous solutions [J].
Bandyopadhyaya, R ;
Nativ-Roth, E ;
Regev, O ;
Yerushalmi-Rozen, R .
NANO LETTERS, 2002, 2 (01) :25-28
[6]   Unusually high thermal conductivity of carbon nanotubes [J].
Berber, S ;
Kwon, YK ;
Tománek, D .
PHYSICAL REVIEW LETTERS, 2000, 84 (20) :4613-4616
[7]   Anomalous thermal conductivity enhancement in nanotube suspensions [J].
Choi, SUS ;
Zhang, ZG ;
Yu, W ;
Lockwood, FE ;
Grulke, EA .
APPLIED PHYSICS LETTERS, 2001, 79 (14) :2252-2254
[8]   Pool boiling characteristics of nano-fluids [J].
Das, SK ;
Putra, N ;
Roetzel, W .
INTERNATIONAL JOURNAL OF HEAT AND MASS TRANSFER, 2003, 46 (05) :851-862
[9]   Heat transfer of aqueous suspensions of carbon nanotubes (CNT nanofluids) [J].
Ding, YL ;
Alias, H ;
Wen, DS ;
Williams, RA .
INTERNATIONAL JOURNAL OF HEAT AND MASS TRANSFER, 2006, 49 (1-2) :240-250
[10]   A new determination of the molecular dimensions [J].
Einstein, A .
ANNALEN DER PHYSIK, 1906, 19 (02) :289-306