Mechanistic model for prediction of structured packing mass transfer performance in CO2 absorption with chemical reactions

被引:45
作者
Aroonwilas, A [1 ]
Tontiwachwuthikul, P [1 ]
机构
[1] Univ Regina, Fac Engn, Proc Syst Lab, Regina, SK S4S 0A2, Canada
基金
加拿大自然科学与工程研究理事会;
关键词
absorption; carbon dioxide; mass transfer; mathematical modelling; packed bed; structured packing;
D O I
10.1016/S0009-2509(00)00035-X
中图分类号
TQ [化学工业];
学科分类号
0817 ;
摘要
A mechanistic model based on liquid irrigation feature is proposed for predicting mass transfer performance of sheet-metal structured packings. The model was used to simulate mass transfer performance of Gempak 4A structured packings for CO2 absorption using NaON aqueous solutions. A very good agreement between the simulation results and the experimental data acquired from a pilot CO2 absorption unit was found under ranges of process parameters including liquid load, initial liquid distribution pattern, and liquid temperature. In comparison with published mass transfer correlations, the proposed model can effectively handle the prediction in a wider range of the liquid load. (C) 2000 Elsevier Science Ltd. All rights reserved.
引用
收藏
页码:3651 / 3663
页数:13
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