Concentration and chemical composition of PM2.5 in Shanghai for a 1-year period

被引:407
作者
Ye, BM
Ji, XL
Yang, HZ
Yao, XH
Chan, CK
Cadle, SH
Chan, T
Mulawa, PA
机构
[1] GM R&D Ctr, Chem & Environm Sci Lab, Warren, MI 48090 USA
[2] Tongji Univ, Sch Environm Sci & Engn, Shanghai 200092, Peoples R China
[3] Hong Kong Univ Sci & Technol, Dept Chem Engn, Hong Kong, Hong Kong, Peoples R China
关键词
particulate matter; PM2.5; composition; Shanghai; China; sources; seasonal variation; AIR-POLLUTION; PULMONARY-FUNCTION; CHINA; PARTICULATE; QUALITY; IMPROVE;
D O I
10.1016/S1352-2310(02)00918-4
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Weekly PM2.5 samples were collected in Shanghai, China at two sites, Tongji University and Hainan Road. Sampling started in March 1999 and was conducted for 1 year. The ambient mass concentration and chemical composition of the PM2.5 were determined. Chemical analyses included elemental composition, water-soluble ions, and organic and elemental carbon. Weekly PM2.5 mass concentrations ranged from 21 to 147 mug/m(3), with annual average concentrations of 57.9 and 61.4 mug/m(3) at the two sites, respectively. Seasonal variation Of PM2.5 concentrations was significant, with the highest concentrations observed from mid-November through December and the lowest from June through September. Ammonium sulfate and nitrate accounted for 41.6% of the PM2.5 mass with sulfate alone accounting for 23.4% of the PM2.5 mass. Carbonaceous material accounted for 41.4% of the PM2.5 mass, with 73% of that mass being organic, as defined by the TOR analysis method. Crustal components averaged 9.6% of the PM2.5 mass. Potassium, which was 95% water soluble, accounted for 2.7% of the PM2.5 mass. (C) 2002 Elsevier Science Ltd. All rights reserved.
引用
收藏
页码:499 / 510
页数:12
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