Passively correcting phase drift in two-dimensional infrared spectroscopy

被引：30

作者：

Ding, Feng ^{[1
]}

Mukherjee, Prabuddha ^{[1
]}

Zanni, Martin T. ^{[1
]}

机构：

[1] Univ Wisconsin, Dept Chem, Madison, WI 53706 USA

来源：

OPTICS LETTERS | 2006年 / 31卷 / 19期

关键词：

D O I：

10.1364/OL.31.002918

中图分类号：

O43 [光学];

学科分类号：

070207 ; 0803 ;

摘要：

Heterodyned two-dimensional (2D) IR spectra often suffer from inaccurate pulse delays and phase drift. We report a passive method of correcting these two inaccuracies by using wedged optics for subfemtosecond pulse delay resolution and reference measurements for phase corrections. Our approach is easy to implement into existing 2D IR spectrometers and makes experiments requiring long-term phase stability possible, such as the collection of 3D IR spectra. (c) 2006 Optical Society of America.

引用

收藏

页码：2918 / 2920

页数：3

相关论文

共 9 条

[1] Phase-stabilized two-dimensional electronic spectroscopy [J].

Brixner, T ;

Mancal, T ;

Stiopkin, IV ;

Fleming, GR .

JOURNAL OF CHEMICAL PHYSICS, 2004, 121 (09) :4221-4236

[2] Ultrafast memory loss and energy redistribution in the hydrogen bond network of liquid H2O [J].

Cowan, ML ;

Bruner, BD ;

Huse, N ;

Dwyer, JR ;

Chugh, B ;

Nibbering, ETJ ;

Elsaesser, T ;

Miller, RJD .

NATURE, 2005, 434 (7030) :199-202

[3] Heterodyned fifth-order 2D-IR spectroscopy of the azide ion in an ionic glass [J].

Fulmer, EC ;

Ding, F ;

Zanni, MT .

JOURNAL OF CHEMICAL PHYSICS, 2005, 122 (03)

[4] Vibrational dynamics of ions in glass from fifth-order two-dimensional infrared spectroscopy [J].

Fulmer, EC ;

Ding, F ;

Mukherjee, P ;

Zanni, MT .

PHYSICAL REVIEW LETTERS, 2005, 94 (06)

[5] Three-dimensional-IR spectroscopy: Beyond the two-point frequency fluctuation correlation function [J].

Hamm, P .

JOURNAL OF CHEMICAL PHYSICS, 2006, 124 (12)

[6]

LOPARO JJ, UNPUB J CHEM PHYS

[7] Theoretical description of the nonlinear response functions associated with eight distinctive three-dimensional vibrational spectroscopies [J].

Park, K ;

Cho, MH .

JOURNAL OF CHEMICAL PHYSICS, 2000, 112 (11) :5021-5036

[8] Infrared analogs of heteronuclear nuclear magnetic resonance coherence transfer experiments in peptides [J].

Scheurer, C ;

Mukamel, S .

JOURNAL OF CHEMICAL PHYSICS, 2002, 116 (15) :6803-6816

[9] Active phase stabilization in Fourier-transform two-dimensional infrared spectroscopy [J].

Volkov, V ;

Schanz, R ;

Hamm, P .

OPTICS LETTERS, 2005, 30 (15) :2010-2012