A new approach to modelling quantum dot concentrators

被引:79
作者
Chatten, AJ [1 ]
Barnham, KWJ
Buxton, BF
Ekins-Daukes, NJ
Malik, MA
机构
[1] Univ London Imperial Coll Sci Technol & Med, Dept Phys, London SW7 2BW, England
[2] UCL, Dept Comp Sci, London WC1E 6BT, England
[3] Univ London Imperial Coll Sci Technol & Med, Dept Chem, London SW7 2AZ, England
基金
英国工程与自然科学研究理事会;
关键词
quantum dots (QDs); concentrator; luminescence; red shift; re-absorption; modelling; thermodynamics; radiative transfer;
D O I
10.1016/S0927-0248(02)00182-4
中图分类号
TE [石油、天然气工业]; TK [能源与动力工程];
学科分类号
0807 ; 0820 ;
摘要
Luminescent collectors have advantages over geometric concentrators in that tracking is unnecessary and both direct and diffuse radiation can be collected. However, development has been limited by the performance of luminescent dyes. We have recently proposed a novel concentrator in which the dyes are replaced by quantum dots (QDs). Advantages over dyes include that the absorption threshold can be tuned by choice of dot diameter, and that the red shift between absorption and luminescence is related to the spread of dot sizes. In this paper we discuss how we have developed a self-consistent thermodynamic model for planar concentrators which allows for re-absorption by the QDs. (C) 2002 Published by Elsevier Science B.V.
引用
收藏
页码:363 / 371
页数:9
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