Ferroelectricity induced by incommensurate-commensurate magnetic phase transition in multiferroic HoMn2O5

被引:37
作者
Kimura, Hiroyuki [1 ]
Kamada, Youichi
Noda, Yukio
Kaneko, Koji
Metokii, Naoto
Kohn, Key
机构
[1] Tohoku Univ, Inst Multidisciplinary Res Adv Mat, Sendai, Miyagi 9808577, Japan
[2] Japan Atom Enrgy Agcy, Adv Sci Res Ctr, Tokai, Ibaraki 3191195, Japan
[3] Waseda Univ, Dept Phys, Tokyo 1698555, Japan
关键词
multiferroics; colossal magnetoelectric effect; neutron diffraction; incommensurate-commensurate magnetic phase transition; ferroelectricity;
D O I
10.1143/JPSJ.75.113701
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
Neutron diffraction measurements under high magnetic fields in multiferroic HoMn2O5 have revealed a clear relationship between microscopic magnetism and field-induced ferroelectricity. The applied magnetic field induces a first-order phase transition from an incommensurate magnetic order to a commensurate magnetic order, where a spontaneous electric polarization occurs. The one-to-one correspondence between the magnetic phase diagram and the dielectric phase diagram under magnetic field clearly indicates that the electric polarization is magnetically induced and the commensurate magnetic structure is indispensable to the ferroelectricity in the multiferroic RMn2O5 system.
引用
收藏
页数:4
相关论文
共 25 条
[1]   CRYSTAL STRUCTURE OF PARAMAGNETIC DYMN2O5 AT 298 DEGREES K [J].
ABRAHAMS, SC ;
BERNSTEIN, JL .
JOURNAL OF CHEMICAL PHYSICS, 1967, 46 (10) :3776-+
[2]   Field-induced linear magnetoelastic coupling in multiferroic TbMnO3 -: art. no. 020102 [J].
Aliouane, N ;
Argyriou, DN ;
Strempfer, J ;
Zegkinoglou, I ;
Landsgesell, S ;
Zimmermann, MV .
PHYSICAL REVIEW B, 2006, 73 (02)
[3]   Collinear to spiral spin transformation without changing the modulation wavelength upon ferroelectric transition in Tb1-xDyxMnO3 [J].
Arima, T ;
Tokunaga, A ;
Goto, T ;
Kimura, H ;
Noda, Y ;
Tokura, Y .
PHYSICAL REVIEW LETTERS, 2006, 96 (09)
[4]   Magnetic-field-induced transition in the lattice modulation of colossal magnetoelectric GdMnO3 and TbMnO3 compounds -: art. no. 100102 [J].
Arima, T ;
Goto, T ;
Yamasaki, Y ;
Miyasaka, S ;
Ishii, K ;
Tsubota, M ;
Inami, T ;
Murakami, Y ;
Tokura, Y .
PHYSICAL REVIEW B, 2005, 72 (10)
[5]   Spin structure and magnetic frustration in multiferroic RMn2O5 (R=Tb,Ho,Dy) -: art. no. 214402 [J].
Blake, GR ;
Chapon, LC ;
Radaelli, PG ;
Park, S ;
Hur, N ;
Cheong, SW ;
Rodríguez-Carvajal, J .
PHYSICAL REVIEW B, 2005, 71 (21)
[6]   Ferroelectricity induced by acentric spin-density waves in YMn2O5 [J].
Chapon, LC ;
Radaelli, PG ;
Blake, GR ;
Park, S ;
Cheong, SW .
PHYSICAL REVIEW LETTERS, 2006, 96 (09)
[7]  
Curie P., 1894, J. Phys. Theor. Appl, V3, P393, DOI DOI 10.1051/JPHYSTAP:018940030039300
[8]   THEORY OF THE ROLE OF COVALENCE IN THE PEROVSKITE-TYPE MANGANITES [LA,M(II)]MNO3 [J].
GOODENOUGH, JB .
PHYSICAL REVIEW, 1955, 100 (02) :564-573
[9]   Magnetic-field-induced polarization and depolarization in HoMn2O5 and ErMn2O5 -: art. no. 064421 [J].
Higashiyama, D ;
Miyasaka, S ;
Tokura, Y .
PHYSICAL REVIEW B, 2005, 72 (06)
[10]   Colossal magnetodielectric effects in DyMn2O5 -: art. no. 107207 [J].
Hur, N ;
Park, S ;
Sharma, PA ;
Guha, S ;
Cheong, SW .
PHYSICAL REVIEW LETTERS, 2004, 93 (10) :107207-1