An Efficient Triple-Junction Polymer Solar Cell Having a Power Conversion Efficiency Exceeding 11%

被引:749
作者
Chen, Chun-Chao [1 ]
Chang, Wei-Hsuan [1 ]
Yoshimura, Ken [2 ]
Ohya, Kenichiro [2 ]
You, Jingbi [1 ]
Gao, Jing [1 ]
Hong, Zirou [1 ]
Yang, Yang [1 ]
机构
[1] Univ Calif Los Angeles, Dept Mat Sci & Engn, Los Angeles, CA 90095 USA
[2] Sumitomo Chem Co Ltd, Tsukuba Mat Dev Lab, Tsukuba, Ibagaki 3003294, Japan
基金
美国国家科学基金会;
关键词
OPEN-CIRCUIT VOLTAGE; LOW-BANDGAP POLYMER; TANDEM POLYMER; DESIGN RULES; FILL FACTOR; PERFORMANCE; LAYER; DONORS;
D O I
10.1002/adma.201402072
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Tandem solar cells have the potential to improve photon conversion efficiencies (PCEs) beyond the limits of single-junction devices. In this study, a triple-junction tandem design is demonstrated by employing three distinct organic donor materials having bandgap energies ranging from 1.4 to 1.9 eV. Through optical modeling, balanced photon absorption rates are achieved and, thereby, the photo currents are matched among the three subcells. Accordingly, an efficient triple-junction tandem organic solar cell can exhibit a record-high PCE of 11.5%.
引用
收藏
页码:5670 / +
页数:9
相关论文
共 50 条
[1]   Triple junction polymer solar cells [J].
Adebanjo, Olusegun ;
Maharjan, Purna P. ;
Adhikary, Prajwal ;
Wang, Mingtai ;
Yang, Shangfeng ;
Qiao, Qiquan .
ENERGY & ENVIRONMENTAL SCIENCE, 2013, 6 (11) :3150-3170
[2]   Hybrid zinc oxide conjugated polymer bulk heterojunction solar cells [J].
Beek, WJE ;
Wienk, MM ;
Kemerink, M ;
Yang, XN ;
Janssen, RAJ .
JOURNAL OF PHYSICAL CHEMISTRY B, 2005, 109 (19) :9505-9516
[3]   Limiting efficiency for current-constrained two-terminal tandem cell stacks [J].
Brown, AS ;
Green, MA .
PROGRESS IN PHOTOVOLTAICS, 2002, 10 (05) :299-307
[4]  
Chang CY, 2013, ADV FUNCT MATER, V23, P5084, DOI [10.1002/adfm201301557, 10.1002/adfm.201301557]
[5]   High-performance semi-transparent polymer solar cells possessing tandem structures [J].
Chen, Chun-Chao ;
Dou, Letian ;
Gao, Jing ;
Chang, Wei-Hsuan ;
Li, Gang ;
Yang, Yang .
ENERGY & ENVIRONMENTAL SCIENCE, 2013, 6 (09) :2714-2720
[6]   Visibly Transparent Polymer Solar Cells Produced by Solution Processing [J].
Chen, Chun-Chao ;
Dou, Letian ;
Zhu, Rui ;
Chung, Choong-Heui ;
Song, Tze-Bin ;
Zheng, Yue Bing ;
Hawks, Steve ;
Li, Gang ;
Weiss, Paul S. ;
Yang, Yang .
ACS NANO, 2012, 6 (08) :7185-7190
[7]   Organic tandem solar cells with complementary absorbing layers and a high open-circuit voltage [J].
Cheyns, D. ;
Rand, B. P. ;
Heremans, P. .
APPLIED PHYSICS LETTERS, 2010, 97 (03)
[8]  
Choi H, 2013, NAT PHOTONICS, V7, P732, DOI [10.1038/nphoton.2013.181, 10.1038/NPHOTON.2013.181]
[9]   Design rules for donors in bulk-heterojunction tandem solar cells-towards 15 % energy-conversion efficiency [J].
Dennler, Gilles ;
Scharber, Markus C. ;
Ameri, Tayebeh ;
Denk, Patrick ;
Forberich, Karen ;
Waldauf, Christoph ;
Brabec, Christoph J. .
ADVANCED MATERIALS, 2008, 20 (03) :579-+
[10]  
DEVOS A, 1980, J PHYS D APPL PHYS, V13, P839, DOI 10.1088/0022-3727/13/5/018