Adsorption of ethene on Cu(111)

被引:30
作者
Linke, R [1 ]
Becker, C [1 ]
Pelster, T [1 ]
Tanemura, M [1 ]
Wandelt, K [1 ]
机构
[1] NAGOYA INST TECHNOL,SHOWA KU,NAGOYA,AICHI 466,JAPAN
关键词
copper; electron energy loss spectroscopy; ethene; low energy electron diffraction; thermal programmed desorption; work function;
D O I
10.1016/S0039-6028(96)01475-6
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The adsorption of ethene on Cu(111) has been investigated using LEED, HREELS, TPD and work function measurements (Delta phi) at 100 K. Ethene adsorption results in a maximum Delta phi value of 0.90 eV. The TPD exhibits a single desorption state with a maximum desorption rate at 120 K. In the vibrational spectrum a dominant energy loss signal at 112 meV is assigned to the out of plane CH2 wagging mode. No additional diffraction pattern could be observed after ethene adsorption in the entire coverage range.
引用
收藏
页码:655 / 658
页数:4
相关论文
共 16 条
[1]   POSITION OF THE SIGMA-SHAPE AND PI-RESONANCES OF C2H2, C2H4 AND C2H6 ON CU(100) AT 60-K - A NEXAFS STUDY [J].
ARVANITIS, D ;
DOBLER, U ;
WENZEL, L ;
BABERSCHKE, K ;
STOHR, J .
SURFACE SCIENCE, 1986, 178 (1-3) :686-692
[2]   ETHYLENE AND ACETYLENE ADSORPTION ON CU(111) AND PT(111) STUDIED BY AUGER-SPECTROSCOPY [J].
CANNING, NDS ;
BAKER, MD ;
CHESTERS, MA .
SURFACE SCIENCE, 1981, 111 (03) :441-451
[3]   A METHOD FOR ESTIMATING SURFACE-REACTION ENERGETICS - APPLICATION TO THE MECHANISM OF ETHYLENE DECOMPOSITION ON PT(111) [J].
CARTER, EA ;
KOEL, BE .
SURFACE SCIENCE, 1990, 226 (03) :339-357
[6]  
Herzberg G., 1945, Molecular Spectra and Molecular Structure: Infrared and Raman of Polyatomic Molecules
[7]  
Ibach H., 1982, ELECT ENERGY LOSS SP
[8]  
IBACH H, 1994, SURF SCI, V299, P129
[9]   EVIDENCE FOR AN UNUSUAL COORDINATION GEOMETRY FOR ETHYLENE ON CU(110) [J].
JENKS, CJ ;
BENT, BE ;
BERNSTEIN, N ;
ZAERA, F .
SURFACE SCIENCE, 1992, 277 (03) :L89-L94
[10]   IRAS STUDIES OF ADSORBED ETHENE (C2H4) ON CLEAN AND OXYGEN-COVERED CU(110) SURFACES [J].
KUBOTA, J ;
KONDO, JN ;
DOMEN, K ;
HIROSE, C .
JOURNAL OF PHYSICAL CHEMISTRY, 1994, 98 (31) :7653-7656