Molecular-field-enhanced optical Kerr effect in absorbing liquids

被引:65
作者
Paparo, D [1 ]
Marrucci, L [1 ]
Abbate, G [1 ]
Santamato, E [1 ]
Kreuzer, M [1 ]
Lehnert, P [1 ]
Vogeler, T [1 ]
机构
[1] TH DARMSTADT,INST PHYS APPL,D-64289 DARMSTADT,GERMANY
关键词
D O I
10.1103/PhysRevLett.78.38
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
A large enhancement of the optical Kerr nonlinearity associated with light-induced molecular orientation is observed in a liquid of anisotropic organic molecules when it is doped with a small amount of dye. The effect is ascribed to a photoinduced intermolecular force field, whose orienting action adds to the direct optical field action. The experimental results are in agreement with a model based on such interpretation. The proposed mechanism is in principle very general, and should work in all absorbing liquids made of anisotropic molecules.
引用
收藏
页码:38 / 41
页数:4
相关论文
共 8 条
[1]  
BOYD RW, 1992, NONLINEAR OPTICS, P178
[2]   MOLECULAR INTERPRETATION OF THE ABSORPTION-INDUCED OPTICAL REORIENTATION OF NEMATIC LIQUID-CRYSTALS [J].
JANOSSY, I .
PHYSICAL REVIEW E, 1994, 49 (04) :2957-2963
[3]   ANOMALOUS OPTICAL FREEDERICKSZ TRANSITION IN AN ABSORBING LIQUID-CRYSTAL [J].
JANOSSY, I ;
LLOYD, AD ;
WHERRETT, BS .
MOLECULAR CRYSTALS AND LIQUID CRYSTALS, 1990, 179 :1-12
[4]   WAVELENGTH DEPENDENCE OF OPTICAL REORIENTATION IN DYE-DOPED NEMATICS [J].
PAPARO, D ;
MADDALENA, P ;
ABBATE, G ;
SANTAMATO, E ;
JANOSSY, I .
MOLECULAR CRYSTALS AND LIQUID CRYSTALS SCIENCE AND TECHNOLOGY SECTION A-MOLECULAR CRYSTALS AND LIQUID CRYSTALS, 1994, 251 :73-84
[5]   Time resolved fluorescence of dye solutions in nematic liquid crystals [J].
Paparo, D ;
Marrucci, L ;
Abbate, G ;
Santamato, E ;
Bartolini, P ;
Torre, R .
MOLECULAR CRYSTALS AND LIQUID CRYSTALS SCIENCE AND TECHNOLOGY SECTION A-MOLECULAR CRYSTALS AND LIQUID CRYSTALS, 1996, 282 :461-472
[6]  
SHEN YR, 1984, PRINCIPLES NONLINEAR, P291
[7]   OPTICAL-FIELD-INDUCED ORDERING IN ISOTROPIC PHASE OF A NEMATIC LIQUID-CRYSTAL [J].
WONG, GKL ;
SHEN, YR .
PHYSICAL REVIEW LETTERS, 1973, 30 (19) :895-897
[8]   STUDY OF PRETRANSITIONAL BEHAVIOR OF LASER-FIELD-INDUCED MOLECULAR ALIGNMENT IN ISOTROPIC NEMATIC SUBSTANCES [J].
WONG, GKL ;
SHEN, YR .
PHYSICAL REVIEW A, 1974, 10 (04) :1277-1284