Glass transition in the polaron dynamics of colossal magnetoresistive manganites

被引:81
作者
Argyriou, DN
Lynn, JW
Osborn, R
Campbell, B
Mitchell, JF
Ruett, U
Bordallo, HN
Wildes, A
Ling, CD
机构
[1] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA
[2] NIST, Ctr Neutron Res, Gaithersburg, MD 20899 USA
[3] Argonne Natl Lab, Intense Pulsed Neutron Source, Argonne, IL 60439 USA
[4] Inst Max Von Laue Paul Langevin, F-38042 Grenoble 09, France
关键词
D O I
10.1103/PhysRevLett.89.036401
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
Neutron scattering measurements on a bilayer manganite near optimal doping show that the short-range polaron correlations are completely dynamic at high T , but then freeze upon cooling to a temperature T*approximate to310 K . This glass transition suggests that the paramagnetic/insulating state arises from an inherent orbital frustration that inhibits the formation of a long-range orbital- and charge-ordered state. Upon further cooling into the ferromagnetic-metallic state (T-C=114 K) , where the polarons melt, the diffuse scattering quickly develops into a propagating, transverse optic phonon.
引用
收藏
页码:364011 / 364014
页数:4
相关论文
共 22 条
[1]   Charge ordering and polaron formation in the magnetoresistive oxide La0.7Ca0.3MnO3 [J].
Adams, CP ;
Lynn, JW ;
Mukovskii, YM ;
Arsenov, AA ;
Shulyatev, DA .
PHYSICAL REVIEW LETTERS, 2000, 85 (18) :3954-3957
[2]   Lattice displacements above TC in the layered manganite La1.2Sr1.8Mn2O7 [J].
Argyriou, DN ;
Bordallo, HN ;
Mitchell, JF ;
Jorgensen, JD ;
Strouse, GF .
PHYSICAL REVIEW B, 1999, 60 (09) :6200-6203
[3]   Charge ordering and phase competition in the layered perovskite LaSr2Mn2O7 [J].
Argyriou, DN ;
Bordallo, HN ;
Campbell, BJ ;
Cheetham, AK ;
Cox, DE ;
Gardner, JS ;
Hanif, K ;
dos Santos, A ;
Strouse, GF .
PHYSICAL REVIEW B, 2000, 61 (22) :15269-15276
[4]   Colossal effects in transition metal oxides caused by intrinsic inhomogeneities [J].
Burgy, J ;
Mayr, M ;
Martin-Mayor, V ;
Moreo, A ;
Dagotto, E .
PHYSICAL REVIEW LETTERS, 2001, 87 (27) :277202-277202
[5]   Structure of nanoscale polaron correlations in La1.2Sr1.8Mn2O7 -: art. no. 014427 [J].
Campbell, BJ ;
Osborn, R ;
Argyriou, DN ;
Vasiliu-Doloc, L ;
Mitchell, JF ;
Sinha, SK ;
Ruett, U ;
Ling, CD ;
Islam, Z ;
Lynn, JW .
PHYSICAL REVIEW B, 2002, 65 (01) :1-5
[6]   Short-range polaron correlations in the ferromagnetic La1-xCaxMnO3 [J].
Dai, PC ;
Fernandez-Baca, JA ;
Wakabayashi, N ;
Plummer, EW ;
Tomioka, Y ;
Tokura, Y .
PHYSICAL REVIEW LETTERS, 2000, 85 (12) :2553-2556
[7]   Glassy statics and dynamics in the chemically ordered pyrochlore anti-ferromagnet Y2Mo2O7 [J].
Gardner, JS ;
Gaulin, BD ;
Lee, SH ;
Broholm, C ;
Raju, NP ;
Greedan, JE .
PHYSICAL REVIEW LETTERS, 1999, 83 (01) :211-214
[8]   THEORY OF THE ROLE OF COVALENCE IN THE PEROVSKITE-TYPE MANGANITES [LA,M(II)]MNO3 [J].
GOODENOUGH, JB .
PHYSICAL REVIEW, 1955, 100 (02) :564-573
[9]   Specific heat of La1.2Sr1.8Mn2O7 [J].
Gordon, JE ;
Bader, SD ;
Mitchell, JF ;
Osborn, R ;
Rosenkranz, S .
PHYSICAL REVIEW B, 1999, 60 (09) :6258-6261
[10]   Temperature and field dependence of the phase separation, structure, and magnetic ordering in La1-xCaxMnO3 (x=0.47, 0.50, and 0.53) [J].
Huang, Q ;
Lynn, JW ;
Erwin, RW ;
Santoro, A ;
Dender, DC ;
Smolyaninova, VN ;
Ghosh, K ;
Greene, RL .
PHYSICAL REVIEW B, 2000, 61 (13) :8895-8905