Entropy balance and evidence for local spin singlets in a Kagome-like magnet

被引:130
作者
Ramirez, AP
Hessen, B
Winklemann, M
机构
[1] Lucent Technol, Bell Labs, Murray Hill, NJ 07974 USA
[2] Univ Groningen, Dept Chem, NL-9747 AG Groningen, Netherlands
[3] Hahn Meitner Inst Kernforsch Berlin GmbH, D-14109 Berlin, Germany
关键词
D O I
10.1103/PhysRevLett.84.2957
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We have measured the specific heat C(T) of the S = 3/2 Kagome-lattice-containing compound SrCr9pGa12-9pO19. We find little field dependence of the low-temperature C(T), consistent with a low-energy spectrum dominated by many-body singlet excitations. At high temperatures, we recover only similar to 50% of the total R ln4 entropy.
引用
收藏
页码:2957 / 2960
页数:4
相关论文
共 21 条
[1]   ANTIFERROMAGNETIC FLUCTUATIONS AND SHORT-RANGE ORDER IN A KAGOME LATTICE [J].
BROHOLM, C ;
AEPPLI, G ;
ESPINOSA, GP ;
COOPER, AS .
PHYSICAL REVIEW LETTERS, 1990, 65 (25) :3173-3176
[2]   QUANTUM SPIN NEMATICS - MOMENT-FREE MAGNETISM [J].
CHANDRA, P ;
COLEMAN, P .
PHYSICAL REVIEW LETTERS, 1991, 66 (01) :100-103
[3]   NUCLEAR ANTIFERROMAGNETISM IN A REGISTERED HE-3 SOLID [J].
ELSER, V .
PHYSICAL REVIEW LETTERS, 1989, 62 (20) :2405-2408
[4]   Cooperative paramagnetism in the geometrically frustrated pyrochlore antiferromagnet Tb2Ti2O7 [J].
Gardner, JS ;
Dunsiger, SR ;
Gaulin, BD ;
Gingras, MJP ;
Greedan, JE ;
Kiefl, RF ;
Lumsden, MD ;
MacFarlane, WA ;
Raju, NP ;
Sonier, JE ;
Swainson, I ;
Tun, Z .
PHYSICAL REVIEW LETTERS, 1999, 82 (05) :1012-1015
[5]   SPIN-GLASS-LIKE BEHAVIOR IN Y2MO2O7, A CONCENTRATED, CRYSTALLINE SYSTEM WITH NEGLIGIBLE APPARENT DISORDER [J].
GREEDAN, JE ;
SATO, M ;
XU, Y ;
RAZAVI, FS .
SOLID STATE COMMUNICATIONS, 1986, 59 (12) :895-897
[6]   Order versus disorder in the quantum Heisenberg antiferromagnet on the kagome lattice using exact spectra analysis [J].
Lecheminant, P ;
Bernu, B ;
Lhuillier, C ;
Pierre, L ;
Sindzingre, P .
PHYSICAL REVIEW B, 1997, 56 (05) :2521-2529
[7]   Isolated spin pairs and two-dimensional magnetism in SrCr9pGa12-9pO19 [J].
Lee, SH ;
Broholm, C ;
Aeppli, G ;
Perring, TG ;
Hessen, B ;
Taylor, A .
PHYSICAL REVIEW LETTERS, 1996, 76 (23) :4424-4427
[8]   MAGNETIC TRANSITION IN HIGHLY FRUSTRATED SRCR8GA4O19 - THE ARCHETYPAL KAGOME SYSTEM [J].
MARTINEZ, B ;
LABARTA, A ;
RODRIGUEZSOLA, R ;
OBRADORS, X .
PHYSICAL REVIEW B, 1994, 50 (21) :15779-15786
[9]   Low-temperature properties of classical geometrically frustrated antiferromagnets [J].
Moessner, R ;
Chalker, JT .
PHYSICAL REVIEW B, 1998, 58 (18) :12049-12062
[10]   MAGNETIC FRUSTRATION AND LATTICE DIMENSIONALITY IN SRCR8GA4O19 [J].
OBRADORS, X ;
LABARTA, A ;
ISALGUE, A ;
TEJADA, J ;
RODRIGUEZ, J ;
PERNET, M .
SOLID STATE COMMUNICATIONS, 1988, 65 (03) :189-192