Dewetting of glassy polymer films

被引:44
作者
Shenoy, V [1 ]
Sharma, A
机构
[1] Indian Inst Sci, Mat Res Ctr, Bangalore 560012, Karnataka, India
[2] Indian Inst Technol, Dept Chem Engn, Kanpur 208016, Uttar Pradesh, India
关键词
D O I
10.1103/PhysRevLett.88.236101
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
Dynamics and morphology of hole growth in a film of power hardening viscoplastic solid [yield stress similar to(strain-rate )(n) ] is investigated. At short times the growth is exponential and depends on the initial hole size. At long times, for n>1/3, the growth is again exponential but with a different exponent. However, for n<1/3 the hole growth slows and the hole radius approaches an asymptotic value at long times. The rim shape is highly asymmetric, the height of which has a power law dependence on the hole radius (exponent close to unity for 0.25<n<0.4 ). The above results explain recent intriguing experiments of Reiter [Phys. Rev. Lett., 87, 186 101 (2001)] on dewetting.
引用
收藏
页码:4 / 236101
页数:4
相关论文
共 15 条
[1]   Dewetting of supported viscoelastic polymer films: Birth of rims [J].
BrochardWyart, F ;
Debregeas, G ;
Fondecave, R ;
Martin, P .
MACROMOLECULES, 1997, 30 (04) :1211-1213
[2]  
CRIST B, 1993, MAT SCI TECHNOLOGY, V12, P427
[3]   Effect of free surfaces on the glass transition temperature of thin polymer films [J].
Forrest, JA ;
DalnokiVeress, K ;
Stevens, JR ;
Dutcher, JR .
PHYSICAL REVIEW LETTERS, 1996, 77 (10) :2002-2005
[4]   Interface and chain confinement effects on the glass transition temperature of thin polymer films [J].
Forrest, JA ;
DalnokiVeress, K ;
Dutcher, JR .
PHYSICAL REVIEW E, 1997, 56 (05) :5705-5716
[5]  
HERMINGHAUS S, CONDMAT0201193
[6]   Growth of holes in liquid films with partial slippage [J].
Jacobs, K ;
Seemann, R ;
Schatz, G ;
Herminghaus, S .
LANGMUIR, 1998, 14 (18) :4961-4963
[7]  
Kawana S, 2001, PHYS REV E, V63, DOI 10.1103/PhysRevE.63.021501
[8]   SIZE-DEPENDENT DEPRESSION OF THE GLASS-TRANSITION TEMPERATURE IN POLYMER-FILMS [J].
KEDDIE, JL ;
JONES, RAL ;
CORY, RA .
EUROPHYSICS LETTERS, 1994, 27 (01) :59-64
[9]  
Khan A S, 1995, Continuum Theory of Plasticity, V1st
[10]   Long-scale evolution of thin liquid films [J].
Oron, A ;
Davis, SH ;
Bankoff, SG .
REVIEWS OF MODERN PHYSICS, 1997, 69 (03) :931-980