Gas-dynamic consideration of the laser evaporation synthesis of single-wall carbon nanotubes

被引:53
作者
Gorbunov, AA [1 ]
Friedlein, R
Jost, O
Golden, MS
Fink, J
Pompe, W
机构
[1] Tech Univ Dresden, Inst Werkstoffwissensch, D-01062 Dresden, Germany
[2] Inst Festkorper & Werkstofforsch, D-01177 Dresden, Germany
来源
APPLIED PHYSICS A-MATERIALS SCIENCE & PROCESSING | 1999年 / 69卷 / Suppl 1期
关键词
D O I
10.1007/s003390051483
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
The abundance of carbon single-wall nanotubes (SWNTs) in soot synthesized by pulsed laser evaporation of graphite is studied over a wide range of synthesis conditions. The derived SWNT growth time-scale appears to be much longer than any characteristic time-scale in a simplified model of the relaxation of a high-pressure hot condensing gas bubble in a background atmosphere. It is concluded that SWNT nucleation and growth take place in relaxed, condensed, thermalized evaporation products at an optimal temperature between 850-1250 degrees C at a rate of few mu m length per second, which is consistent with a condensed state "precipitation" mechanism for the SWNT formation.
引用
收藏
页码:S593 / S596
页数:4
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