Active centres on vanadia-based catalysts for selective oxidation of hydrocarbons

被引:85
作者
GrzybowskaSwierkosz, B
机构
[1] Inst. of Catalys. and Surf. Chem., Polish Academy of Sciences
关键词
vanadia-based catalysts; selective oxidation; hydrocarbons;
D O I
10.1016/S0926-860X(97)00115-4
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
On the basis of the papers presented in this issue the structure of active centres for different steps of selective oxidation of hydrocarbons on vanadia-based catalysts has been discussed. The physicochemical properties of the vanadia-based catalysts, which control the selectivity to products of oxidative dehydrogenation vs. that to oxygenated products in the oxidation reactions, have also been considered.
引用
收藏
页码:409 / 420
页数:12
相关论文
共 33 条
[1]   A MOLECULAR-LEVEL MECHANISM OF N-BUTANE OXIDATION TO MALEIC-ANHYDRIDE OVER VANADYL PYROPHOSPHATE [J].
AGASKAR, PA ;
DECAUL, L ;
GRASSELLI, RK .
CATALYSIS LETTERS, 1994, 23 (3-4) :339-351
[2]   OXIDATION ACTIVITY AND ACID-BASE PROPERTIES OF MIXED-OXIDE CATALYSTS CONTAINING TITANIA .1. TIO-2-MOO-3 AND TIO-2-V-2O-5 SYSTEMS [J].
AI, M .
BULLETIN OF THE CHEMICAL SOCIETY OF JAPAN, 1976, 49 (05) :1328-1334
[3]   INFLUENCE OF GRAIN MORPHOLOGY OF V2O5 ON ITS REDUCIBILITY AND SELECTIVITY FOR METHANOL OXIDATION [J].
BAIKER, A ;
MONTI, D .
JOURNAL OF CATALYSIS, 1985, 91 (02) :361-365
[4]  
Bielanski A., 1991, OXYGEN CATALYSIS, DOI DOI 10.1201/9781482293289
[5]   N-BUTANE SELECTIVE OXIDATION ON VANADIUM-BASED OXIDES - DEPENDENCE ON CATALYST MICROSTRUCTURE [J].
BUSCA, G ;
CENTI, G ;
TRIFIRO, F .
APPLIED CATALYSIS, 1986, 25 (1-2) :265-272
[6]   SURFACE-ACIDITY OF VANADYL PYROPHOSPHATE, ACTIVE PHASE IN NORMAL-BUTANE SELECTIVE OXIDATION [J].
BUSCA, G ;
CENTI, G ;
TRIFIRO, F ;
LORENZELLI, V .
JOURNAL OF PHYSICAL CHEMISTRY, 1986, 90 (07) :1337-1344
[7]  
BUSCA G, 1994, STUD SURF SCI CATAL, V82, P253
[8]   A SELECTIVITY FACTOR IN VAPOR-PHASE HYDROCARBON OXIDATION CATALYSIS [J].
CALLAHAN, JL ;
GRASSELLI, RK .
AICHE JOURNAL, 1963, 9 (06) :755-760
[9]   VANADYL PYROPHOSPHATE CATALYSTS - PREFACE [J].
CENTI, G .
CATALYSIS TODAY, 1993, 16 (01) :1-4
[10]   SELECTIVE OXIDATIVE DEHYDROGENATION OF BUTANE OVER V-MG-O CATALYSTS [J].
CHAAR, MA ;
PATEL, D ;
KUNG, MC ;
KUNG, HH .
JOURNAL OF CATALYSIS, 1987, 105 (02) :483-498