Evidence for resonant magnetic tunneling of rare-earth ions: from insulating to metallic matrix

被引:16
作者
Barbara, B
Giraud, R
Wernsdorfer, W
Mailly, D
Lejay, P
Tkachuk, A
Suzuki, H
机构
[1] CNRS, Lab Louis Neel, F-38042 Grenoble 09, France
[2] CNRS, Lab Photon & Nanostruct, Marcoussis, France
[3] CNRS, Ctr Rech Tres Basses Temp, F-38042 Grenoble, France
[4] All Russia SI Vavilov State Opt Inst, St Petersburg 199034, Russia
[5] NIMS, Nanomat Lab, Tsukuba, Ibaraki 3050047, Japan
关键词
quantum tunneling; entanglement; rare-earth; impurities;
D O I
10.1016/j.jmmm.2003.12.654
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
Tunneling of the total angular momentum of Ho3+ in LiYF4 (insulating matrix) is demonstrated. Due to strong hyperfine interactions, electronic angular momentum and nuclear spin tunnel simultaneously (two-body entanglement) and due to weak dipolar interactions, pairs of Ho3+ ions also tunnel simultaneously (four-body entanglement). Similar results obtained with a metallic matrix (YRu2Si2) prove the persistence of tunneling in the presence of free carriers. (C) 2003 Elsevier B.V. All rights reserved.
引用
收藏
页码:1024 / 1029
页数:6
相关论文
共 23 条
[1]   ISOTOPE STRUCTURE IN OPTICAL-SPECTRA OF LIYF4-HO3+ [J].
AGLADZE, NI ;
POPOVA, MN ;
ZHIZHIN, GN ;
EGOROV, VJ ;
PETROVA, MA .
PHYSICAL REVIEW LETTERS, 1991, 66 (04) :477-480
[2]   MESOSCOPIC QUANTUM TUNNELING OF THE MAGNETIZATION [J].
BARBARA, B ;
WERNSDORFER, W ;
SAMPAIO, LC ;
PARK, JG ;
PAULSEN, C ;
NOVAK, MA ;
FERRE, R ;
MAILLY, D ;
SESSOLI, R ;
CANESCHI, A ;
HASSELBACH, K ;
BENOIT, A ;
THOMAS, L .
JOURNAL OF MAGNETISM AND MAGNETIC MATERIALS, 1995, 140 :1825-1828
[3]   MACROSCOPIC QUANTUM TUNNELING IN ANTIFERROMAGNETS [J].
BARBARA, B ;
CHUDNOVSKY, EM .
PHYSICS LETTERS A, 1990, 145 (04) :205-208
[4]   Condensed-matter physics - Two bodies are better than one [J].
Barbara, B .
NATURE, 2003, 421 (6918) :32-33
[5]   CROSS-RELAXATION IN SPIN SYSTEMS [J].
BLOEMBERGEN, N ;
SHAPIRO, S ;
PERSHAN, PS ;
ARTMAN, JO .
PHYSICAL REVIEW, 1959, 114 (02) :445-459
[6]   Macroscopic measurement of resonant magnetization tunneling in high-spin molecules [J].
Friedman, JR ;
Sarachik, MP ;
Tejada, J ;
Ziolo, R .
PHYSICAL REVIEW LETTERS, 1996, 76 (20) :3830-3833
[7]  
Gifeisman Sh. N., 1978, Optics and Spectroscopy, V44, P68
[8]   Nuclear spin driven quantum relaxation in LiY0.998Ho0.002F4 -: art. no. 057203 [J].
Giraud, R ;
Wernsdorfer, W ;
Tkachuk, AM ;
Mailly, D ;
Barbara, B .
PHYSICAL REVIEW LETTERS, 2001, 87 (05) :57203-1
[9]  
GIRAUD R, 2002, THESIS J FOURIER U G
[10]   DIFFERENTIAL MAGNETIC SUSCEPTIBILITY OF H0CL3 ,HO(Y)CL3 AND HO(LA)CL3 AT LIQUID-HELIUM TEMPERATURES - OBSERVATION OF A PHONON-BOTTLENECK IN HO(LA)CL3 [J].
HELLWEGE, KH ;
KOTZLER, J ;
WEBER, G .
ZEITSCHRIFT FUR PHYSIK, 1968, 217 (04) :373-&