Field measurements and size-resolved model simulations of turbulent particle transport to a forest canopy

被引:21
作者
Held, Andreas [1 ]
Nowak, Andreas
Wiedensohler, Alfred
Klemm, Otto
机构
[1] Univ Munster, Inst Landscape Ecol, ILOK, D-48149 Munster, Germany
[2] Inst Tropospher Res, IfT, D-04318 Leipzig, Germany
关键词
turbulent particle number flux; particle mass flux; particle deposition model; particle size distribution; effective deposition diameter;
D O I
10.1016/j.jaerosci.2005.06.005
中图分类号
TQ [化学工业];
学科分类号
0817 ;
摘要
Direct measurements of turbulent particle number fluxes above a Norway spruce forest are compared with a size-resolved particle deposition model in combination with particle size distribution measurements. In most cases, the model output is in reasonable agreement with the eddy covariance measurements. The combination of deposition model and size distribution measurements allows the evaluation of size-resolved particle number and mass fluxes. While turbulent particle number fluxes are dominated by ultrafine particles below 50 nm diameter, submicron particle mass fluxes are established mainly in the accumulation mode. The effective deposition diameter D-ed is introduced as a new parameter to describe the effect of the size distribution of a polydisperse particle population on the integral particle transfer velocity. (c) 2005 Elsevier Ltd. All rights reserved.
引用
收藏
页码:786 / 798
页数:13
相关论文
共 22 条
[1]   Design of a DMA-based size spectrometer for a large particle size range and stable operation [J].
Birmili, W ;
Stratmann, F ;
Wiedensohler, A .
JOURNAL OF AEROSOL SCIENCE, 1999, 30 (04) :549-553
[2]   Analysis of measurement techniques to determine dry deposition velocities of aerosol particles with diameters less than 100 nm [J].
Buzorius, G ;
Rannikb, Ü ;
Nilsson, ED ;
Vesala, T ;
Kulmala, M .
JOURNAL OF AEROSOL SCIENCE, 2003, 34 (06) :747-764
[3]   Vertical aerosol particle fluxes measured by eddy covariance technique using condensational particle counter [J].
Buzorius, G ;
Rannik, U ;
Makela, JM ;
Vesala, T ;
Kulmala, M .
JOURNAL OF AEROSOL SCIENCE, 1998, 29 (1-2) :157-171
[4]  
FOKEN T, 2003, ANGEWANDTE METEOROLO
[5]   Measurements and parameterizations of small aerosol deposition velocities to grassland, arable crops, and forest: Influence of surface roughness length on deposition [J].
Gallagher, MW ;
Nemitz, E ;
Dorsey, JR ;
Fowler, D ;
Sutton, MA ;
Flynn, M ;
Duyzer, J .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2002, 107 (D12)
[6]   Observations of particle formation and growth in a mountainous forest region in central Europe [J].
Held, A ;
Nowak, A ;
Birmili, W ;
Wiedensohler, A ;
Forkel, R ;
Klemm, O .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2004, 109 (D23) :1-9
[7]  
HELD A, 2005, UNPUB ATMOSPHERIC EN
[8]  
KLEMM O, 2005, UNPUB ATMOSPHERIC EN
[9]   Formation and growth rates of ultrafine atmospheric particles:: a review of observations [J].
Kulmala, M ;
Vehkamäki, H ;
Petäjä, T ;
Dal Maso, M ;
Lauri, A ;
Kerminen, VM ;
Birmili, W ;
McMurry, PH .
JOURNAL OF AEROSOL SCIENCE, 2004, 35 (02) :143-176
[10]  
Matzner E., 2004, BIOGEOCHEMISTRY FORE