Doubly-resonant sum-frequency generation spectroscopy for surface studies

被引:104
作者
Raschke, MB
Hayashi, M
Lin, SH
Shen, YR
机构
[1] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA
[2] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA
[3] Natl Taiwan Univ, Ctr Condensed Matter Sci, Taipei 10764, Taiwan
[4] Acad Sinica, Inst Atom & Mol Sci, Taipei 10764, Taiwan
关键词
D O I
10.1016/S0009-2614(02)00560-2
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Doubly-resonant infrared visible sum-frequency generation (DR-SFG) as a two-dimensional surface spectroscopy was demonstrated experimentally for the first time. Probing electronic and vibrational transitions of a surface molecular monolayer simultaneously, the technique gives access to information about the electron-vibration coupling of the surface molecules. It allows selective studies of any interface accessible by light. (C) 2002 Elsevier Science B.V. All rights reserved.
引用
收藏
页码:367 / 372
页数:6
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