Ultrafast transient absorption spectroscopy of the hydrated electron: A theory

被引:37
作者
Bratos, S
Leicknam, JC
机构
[1] Lab. de Phys. Theorique des Liquides, Univ. Pierre et Marie Curie, 75252 Paris Cedex 05, Case Courrier 121
关键词
D O I
10.1016/0009-2614(96)00930-X
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
A theory is proposed to study ultrafast transient absorption of the hydrated electron. This theory is a statistical theory using a correlation function description of the nonlinear optical processes involved. Time- and frequency-resolved spectra are examined for both coherent and incoherent incident fields. The nonmonotonic behavior of spectral transients is studied in detail.
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页码:117 / 122
页数:6
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