FT-IR study of Au/Fe2O3 catalysts for CO oxidation at low temperature

被引:176
作者
Minico, S [1 ]
Scire, S [1 ]
Crisafulli, C [1 ]
Visco, AM [1 ]
Galvagno, S [1 ]
机构
[1] UNIV CATANIA,DIPARTIMENTO SCI CHIM,I-95125 CATANIA,ITALY
关键词
CO oxidation; gold; FT-IR spectroscopy;
D O I
10.1023/A:1019081727173
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Coprecipitated Au/Fe2O3 catalysts used for low-temperature catalytic oxidation of carbon monoxide have been studied by FT-IR spectroscopy of adsorbed CO. The FT-IR results have shown that after preparation and exposure to a CO/O-2 mixture gold is present on the surface mainly as Au1+ and Au-0 species. It has been found that in the CO oxidation Au1+ is more active and less stable than Au-0.
引用
收藏
页码:273 / 276
页数:4
相关论文
共 19 条
  • [1] THE OXIDATION AND SCRAMBLING OF CO WITH OXYGEN AT ROOM-TEMPERATURE ON AU/ZNO
    BOCCUZZI, F
    CHIORINO, A
    TSUBOTA, S
    HARUTA, M
    [J]. CATALYSIS LETTERS, 1994, 29 (1-2) : 225 - 234
  • [2] FTIR study of carbon monoxide oxidation and scrambling at room temperature over gold supported on ZnO and TiO2 .2.
    Boccuzzi, F
    Chiorino, A
    Tsubota, S
    Haruta, M
    [J]. JOURNAL OF PHYSICAL CHEMISTRY, 1996, 100 (09) : 3625 - 3631
  • [3] A kinetic and DRIFTS study of low-temperature carbon monoxide oxidation over Au-TiO2 catalysts
    Bollinger, MA
    Vannice, MA
    [J]. APPLIED CATALYSIS B-ENVIRONMENTAL, 1996, 8 (04) : 417 - 443
  • [4] PREPARATION AND CATALYTIC BEHAVIOR OF SUBNANOMETER GOLD DEPOSITED ON TIO2 BY VACUUM CALCINATION
    CUNNINGHAM, D
    TSUBOTA, S
    KAMIJO, N
    HARUTA, M
    [J]. RESEARCH ON CHEMICAL INTERMEDIATES, 1993, 19 (01) : 1 - 13
  • [5] REDUCTIVE CARBONYLATION OF GOLD(III) CHLORIDE
    DELLAMICO, DB
    CALDERAZZO, F
    MARCHETTI, F
    [J]. JOURNAL OF THE CHEMICAL SOCIETY-DALTON TRANSACTIONS, 1976, (18): : 1829 - 1831
  • [6] HALOGENOCARBONYL COMPLEXES OF GOLD
    DELLAMICO, DB
    CALDERAZZO, F
    ROBINO, P
    SEGRE, A
    [J]. JOURNAL OF THE CHEMICAL SOCIETY-DALTON TRANSACTIONS, 1991, (11): : 3017 - 3020
  • [7] COMPARISON OF THE PERFORMANCE-CHARACTERISTICS OF PT/SNOX AND AU/MNOX CATALYSTS FOR LOW-TEMPERATURE CO OXIDATION
    GARDNER, SD
    HOFLUND, GB
    UPCHURCH, BT
    SCHRYER, DR
    KIELIN, EJ
    SCHRYER, J
    [J]. JOURNAL OF CATALYSIS, 1991, 129 (01) : 114 - 120
  • [8] Gold and iron oxide associations under supergene conditions: An experimental approach
    Greffie, C
    Benedetti, MF
    Parron, C
    Amouric, M
    [J]. GEOCHIMICA ET COSMOCHIMICA ACTA, 1996, 60 (09) : 1531 - 1542
  • [9] LOW-TEMPERATURE OXIDATION OF CO OVER GOLD SUPPORTED ON TIO2, ALPHA-FE2O3, AND CO3O4
    HARUTA, M
    TSUBOTA, S
    KOBAYASHI, T
    KAGEYAMA, H
    GENET, MJ
    DELMON, B
    [J]. JOURNAL OF CATALYSIS, 1993, 144 (01) : 175 - 192
  • [10] GOLD CATALYSTS PREPARED BY COPRECIPITATION FOR LOW-TEMPERATURE OXIDATION OF HYDROGEN AND OF CARBON-MONOXIDE
    HARUTA, M
    YAMADA, N
    KOBAYASHI, T
    IIJIMA, S
    [J]. JOURNAL OF CATALYSIS, 1989, 115 (02) : 301 - 309