Critical assessment of the current state of scientific knowledge, terminology, and research needs concerning the role of organic aerosols in the atmosphere, climate, and global change

被引:368
作者
Fuzzi, S. [1 ]
Andreae, M. O.
Huebert, B. J.
Kulmala, M.
Bond, T. C.
Boy, M.
Doherty, S. J.
Guenther, A.
Kanakidou, M.
Kawamura, K.
Kerminen, V. -M.
Lohmann, U.
Russell, L. M.
Poeschl, U.
机构
[1] CNR, Ist Sci Atmosfera & Clima, I-40129 Bologna, Italy
[2] Max Planck Inst Chem, Biogeochem Dept, D-55128 Mainz, Germany
[3] Univ Hawaii, Dept Oceanog, Honolulu, HI 96822 USA
[4] Univ Helsinki, Dept Phys Sci, FIN-00014 Helsinki, Finland
[5] Univ Illinois, Dept Civil & Environm Engn, Urbana, IL 61801 USA
[6] IGAC Core Project Off, Seattle, WA 98115 USA
[7] Natl Ctr Atmospher Res, Div Atmospher Chem, Boulder, CO 80307 USA
[8] Univ Crete, Dept Chem, Environm Chem Proc Lab, Iraklion 71409, Greece
[9] Hokkaido Univ, Inst Low Temp Sci, Sapporo, Hokkaido 0600819, Japan
[10] Finnish Meteorol Inst, Helsinki 00810, Finland
[11] ETH, Inst Atmospher & Climate Sci, CH-8093 Zurich, Switzerland
[12] Univ Calif San Diego, Scripps Inst Oceanog, La Jolla, CA 92093 USA
[13] Tech Univ Munich, Inst Hydrochem, D-81377 Munich, Germany
关键词
D O I
10.5194/acp-6-2017-2006
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
In spite of impressive advances in recent years, our present understanding of organic aerosol (OA) composition, physical and chemical properties, sources and transformation characteristics is still rather limited, and their environmental effects remain highly uncertain. This paper discusses and prioritizes issues related to organic aerosols and their effects on atmospheric processes and climate, providing a basis for future activities in the field. Four main topical areas are addressed: i) sources of OA; ii) formation transformation and removal of OA; iii) physical, chemical and mixing state of OA; iv) atmospheric modelling of OA. Key questions and research priorities regarding these four areas are synthesized in this paper, and outstanding issues for future research are presented for each topical area. In addition, an effort is made to formulate a basic set of consistent and universally applicable terms and definitions for coherent description of atmospheric OA across different scales and disciplines.
引用
收藏
页码:2017 / 2038
页数:22
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