Dark resonances for ground-state transfer of molecular quantum gases

被引:39
作者
Mark, M. J. [1 ,2 ]
Danzl, J. G. [1 ,2 ]
Haller, E. [1 ,2 ]
Gustavsson, M. [1 ,2 ]
Bouloufa, N. [3 ]
Dulieu, O. [3 ]
Salami, H. [4 ]
Bergeman, T. [4 ]
Ritsch, H. [2 ,5 ]
Hart, R. [1 ,2 ]
Naegerl, H. -C. [1 ,2 ]
机构
[1] Univ Innsbruck, Inst Expt Phys, A-6020 Innsbruck, Austria
[2] Univ Innsbruck, Zentrum Quantenphys, A-6020 Innsbruck, Austria
[3] Univ Paris 11, CNRS, Aime Cotton Lab, F-91405 Orsay, France
[4] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA
[5] Univ Innsbruck, Inst Theoret Phys, A-6020 Innsbruck, Austria
来源
APPLIED PHYSICS B-LASERS AND OPTICS | 2009年 / 95卷 / 02期
关键词
POPULATION TRANSFER; POLAR-MOLECULES; ULTRACOLD; PHOTOASSOCIATION; SPECTROSCOPY; ATOMS; CS-2; K-2;
D O I
10.1007/s00340-009-3407-1
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
One possible way to produce ultra-cold, high-phase-space-density quantum gases of molecules in the rovibronic ground state is given by molecule association from quantum-degenerate atomic gases on a Feshbach resonance and subsequent coherent optical multi-photon transfer into the rovibronic ground state. In ultra-cold samples of Cs-2 molecules, we observe two-photon dark resonances that connect the intermediate rovibrational level vertical bar v=73,J=2 > with the rovibrational ground state vertical bar v=0,J=0 > of the singlet X (1) I pound (g) (+) ground-state potential. For precise dark resonance spectroscopy we exploit the fact that it is possible to efficiently populate the level vertical bar v=73,J=2 > by two-photon transfer from the dissociation threshold with the stimulated Raman adiabatic passage (STIRAP) technique. We find that at least one of the two-photon resonances is sufficiently strong to allow future implementation of coherent STIRAP transfer of a molecular quantum gas to the rovibrational ground state vertical bar v=0,J=0 >.
引用
收藏
页码:219 / 225
页数:7
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