Effect of ceramic industrial particulate emission control on key components of ambient PM10

被引:41
作者
Cruz Minguillon, Maria [1 ,2 ]
Monfort, Eliseo [2 ]
Querol, Xavier [1 ]
Alastuey, Andres [1 ]
Celades, Irina [2 ]
Vicente Miro, Jose [3 ]
机构
[1] CSIC, Inst Environm Assessment & Water Res IDAEA, ES-08034 Barcelona, Spain
[2] Univ Jaume 1, Inst Tecnol Ceram, Castellon de La Plana 12006, Spain
[3] Conselleria Medio Ambiente Agua Urbanismo & Vivie, Valencia 46011, Spain
关键词
Emission control; PM10; Ceramics; Effect; BAT; Zinc; Arsenic; Lead; Caesium; Thallium; ABATEMENT TECHNOLOGY; SPAIN; AREA; IMPLEMENTATION; STRATEGIES; DEPOSITION; REMOVAL; IMPACT;
D O I
10.1016/j.jenvman.2009.01.016
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
The relationship between specific particulate emission control and ambient levels of some PM10 components (Zn, As, Pb, Cs, Tl) was evaluated. To this end, the industrial area of Castellon (Eastern Spain) was selected, where around 40% of the EU glazed ceramic tiles and a high proportion of EU ceramic frits are produced. The PM10 emissions from the ceramic processes were calculated over the period 2000-2006, taking into account the degree of implementation of corrective measures throughout the study period. Abatement systems were implemented in the majority of the fusion kilns for frit manufacture in the area as a result of the application of the Directive 1996/61/EC, leading to a marked decrease in PM10 emissions. By contrast, emissions from tile manufacture remained relatively constant because of the few changes in the implementation of corrective measures. On the other hand, ambient PM10 levels and composition measurements were carried out from 2002 to 2006. A high correlation between PM10 emissions from frit manufacture and ambient levels of Zn, As, Pb and Cs (R-2 from 0.61 to 0.98) was observed. On the basis of these results, the potential impact of the implementation of corrective measures to reduce emissions from tile manufacture was quantified, resulting in a possible decrease of 3-5 mu g/m(3) and 2 mu g/m(3) in ambient mineral PM10 (on an annual basis) in urban and suburban areas, respectively. This relatively simple methodology allows us to estimate the direct effect of a reduction in primary particulate emissions on ambient levels of key particulate components, and to make a preliminary quantification of the possibilities of air quality improvement by means of further emission reduction. Therefore, it is a useful tool for developing future air quality plans in the study area and in other industrialised areas. (C) 2009 Elsevier Ltd. All rights reserved.
引用
收藏
页码:2558 / 2567
页数:10
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