Co-current and counter-current modes for methanol steam reforming membrane reactor: Experimental study

被引：50

作者：

Basile, A.

Tosti, S.

Capannelli, G.

Vitulli, G.

Iulianelli, A.

Gallucci, F.

Drioli, E.

机构：

[1] Univ Calabria, ITM, CNR, Inst Membrane Technol, I-87030 Arcavacata Di Rende, CS, Italy

[2] CR ENEA Frascati, Unita Tecn Sci Fus, I-00044 Frascati, Italy

[3] Univ Genoa, Dipartimento Chim & Chim Ind, I-16146 Genoa, Italy

[4] Univ Pisa, CNR, ICCOM, I-50126 Pisa, Italy

[5] Univ Calabria, Dept Chem Engn & Mat, I-87030 Arcavacata Di Rende, CS, Italy

来源：

CATALYSIS TODAY | 2006年 / 118卷 / 1-2期

关键词：

methanol; steam reforming; hydrogen; catalyst; membrane reactor; counter-current mode;

D O I：

10.1016/j.cattod.2006.05.086

中图分类号：

O69 [应用化学];

学科分类号：

081704 ;

摘要：

The methanol steam reforming (MSR) reaction to produce hydrogen was studied from an experimental point of view in membrane reactors (MRs). In order to investigate the behaviour of methanol conversion, the influence of the membrane characteristics, the sweep gas flow rate, as well as the influence of the operating temperature and the different flux configurations were analysed. Experimental results, in terms of methanol conversion as well as hydrogen production and gases selectivity in MRs and a traditional reactor (TR), are proposed. A set of values of key parameters to obtain the maximum hydrogen production is given. (c) 2006 Elsevier B.V All rights reserved.

引用

页码：237 / 245

页数：9

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