The mechanism model of gas-liquid mass transfer enhancement by fine catalyst particles

被引:17
作者
Zhang Junmei
Xu Chunjian [1 ]
Zhou Ming
机构
[1] Tianjin Univ, Res Ctr Chem Engn, Sch Chem Engn & Technol, Tianjin 300072, Peoples R China
[2] Qingdao Univ Sci & Technol, Coll Chem Engn, Qingdao 266042, Peoples R China
关键词
gas-liquid mass transfer; enhancement; three-dimensional model; catalyst particle;
D O I
10.1016/j.cej.2006.03.029
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
In order to present the enhancement of gas-liquid mass transfer by heterogeneous chemical reaction near interface, the mechanism model has been proposed to describe the mass transfer rate for a gas-liquid-solid system containing fine catalyst particles. The composite grid technique has been used to solve the model equations. With this model the effect of particle size, first-order reaction rate constant, distance of particle to gas-liquid interface and residence time of particle near gas-liquid interface on the mass transfer enhancement have been discussed. The particle-particle interaction and slurry apparent viscosity can be considered in the model. The experimental data have been used to verify the model, and the agreement has been found to be satisfied. (c) 2006 Elsevier B.V. All rights reserved.
引用
收藏
页码:149 / 156
页数:8
相关论文
共 20 条
[1]   COMMENTS ON GAS-ABSORPTION WITH CATALYTIC REACTION [J].
ALPER, E ;
DECKWER, WD .
CHEMICAL ENGINEERING SCIENCE, 1981, 36 (06) :1097-1099
[2]   MASS-TRANSFER IN GAS-LIQUID SLURRY REACTORS [J].
BEENACKERS, AACM ;
VANSWAAIJ, WPM .
CHEMICAL ENGINEERING SCIENCE, 1993, 48 (18) :3109-3139
[3]   A one-dimensional instationary heterogeneous mass transfer model for gas absorption in multiphase systems [J].
Brilman, DWF ;
van Swaaij, WPM ;
Versteeg, GF .
CHEMICAL ENGINEERING AND PROCESSING-PROCESS INTENSIFICATION, 1998, 37 (06) :471-488
[4]   Heterogeneous mass transfer models for gas absorption in multiphase systems [J].
Brilman, DWF ;
Goldschmidt, MJV ;
Versteeg, GF ;
van Swaaij, WPM .
CHEMICAL ENGINEERING SCIENCE, 2000, 55 (15) :2793-2812
[5]  
CAI WF, 2003, THESIS TIANJIN U TIA
[6]   COMPOSITE OVERLAPPING MESHES FOR THE SOLUTION OF PARTIAL-DIFFERENTIAL EQUATIONS [J].
CHESSHIRE, G ;
HENSHAW, WD .
JOURNAL OF COMPUTATIONAL PHYSICS, 1990, 90 (01) :1-64
[7]   ABSORPTION OF ISOBUTYLENE IN AQUEOUS SOLUTIONS OF SULPHURIC ACID [J].
GEHLAWAT, JK ;
SHARMA, MM .
CHEMICAL ENGINEERING SCIENCE, 1968, 23 (10) :1173-&
[8]   THE ABSORPTION OF GASES IN AQUEOUS ACTIVATED CARBON SLURRIES ENHANCED BY ADSORBING OR CATALYTIC PARTICLES [J].
HOLSTVOOGD, RD ;
VANSWAAIJ, WPM ;
VANDIERENDONCK, LL .
CHEMICAL ENGINEERING SCIENCE, 1988, 43 (08) :2181-2187
[9]   PENETRATION MODEL FOR GAS-ABSORPTION WITH REACTION IN A SLURRY CONTAINING FINE INSOLUBLE PARTICLES [J].
HOLSTVOOGD, RD ;
PTASINSKI, KJ ;
VANSWAAIJ, WPM .
CHEMICAL ENGINEERING SCIENCE, 1986, 41 (04) :867-873
[10]   OXYGEN-TRANSFER ENHANCEMENT IN AQUEOUS PERFLUOROCARBON FERMENTATION SYSTEMS .2. THEORETICAL-ANALYSIS [J].
JUNKER, BH ;
WANG, DIC ;
HATTON, TA .
BIOTECHNOLOGY AND BIOENGINEERING, 1990, 35 (06) :586-597