Strong coupling between surface plasmons and excitons in an organic semiconductor

被引：677

作者：

Bellessa, J ^{[1
]}

Bonnand, C

Plenet, JC

Mugnier, J

机构：

[1] Univ Lyon 1, CNRS, UMR 5586, Lab Phys Mat Condensee & Nanostruct, F-69622 Villeurbanne, France

[2] Univ Lyon 1, CNRS, UMR 5620, Lab Physicochim Mat Luminescents, F-69622 Villeurbanne, France

来源：

PHYSICAL REVIEW LETTERS | 2004年 / 93卷 / 03期

关键词：

D O I：

10.1103/PhysRevLett.93.036404

中图分类号：

O4 [物理学];

学科分类号：

0702 ;

摘要：

We report on the observation of a strong coupling between a surface plasmon and an exciton. Reflectometry experiments are performed on an organic semiconductor, namely, cyanide dye J aggregates, deposited on a silver film. The dispersion lines present an anticrossing that is the signature of a strong plasmon-exciton coupling. Mixed states are formed in a similar way as microcavities polaritons. The Rabi splitting characteristic of this coupling reaches 180 meV at room temperature. The emission of the low energy plasmon-exciton mixed state has been observed and is largely shifted from the uncoupled emission.

引用

页码：036404 / 1

页数：4

共 18 条

[1] Cavity polaritons in microcavities containing disordered organic semiconductors [J].

Agranovich, VM ;

Litinskaia, M ;

Lidzey, DG .

PHYSICAL REVIEW B, 2003, 67 (08)

[2]

Drexhage K. H., 1974, PROGR OPTICS, V12

[3] TIME-DEPENDENT DECAY OF SURFACE-PLASMON-COUPLED MOLECULAR FLUORESCENCE [J].

EAGEN, CF ;

WEBER, WH ;

MCCARTHY, SL ;

TERHUNE, RW .

CHEMICAL PHYSICS LETTERS, 1980, 75 (02) :274-277

[4] Strong exciton-photon coupling in a low-Q all-metal mirror microcavity [J].

Hobson, PA ;

Barnes, WL ;

Lidzey, DG ;

Gehring, GA ;

Whittaker, DM ;

Skolnick, MS ;

Walker, S .

APPLIED PHYSICS LETTERS, 2002, 81 (19) :3519-3521

[5] RADIATIVE DECAY OF NON RADIATIVE SURFACE PLASMONS EXCITED BY LIGHT [J].

KRETSCHM.E ;

RAETHER, H .

ZEITSCHRIFT FUR NATURFORSCHUNG PART A-ASTROPHYSIK PHYSIK UND PHYSIKALISCHE CHEMIE, 1968, A 23 (12) :2135-&

[6] Strong exciton-photon coupling in an organic semiconductor microcavity [J].

Lidzey, DG ;

Bradley, DDC ;

Skolnick, MS ;

Virgili, T ;

Walker, S ;

Whittaker, DM .

NATURE, 1998, 395 (6697) :53-55

[7] Room temperature polariton emission from strongly coupled organic semiconductor microcavities [J].

Lidzey, DG ;

Bradley, DDC ;

Virgili, T ;

Armitage, A ;

Skolnick, MS ;

Walker, S .

PHYSICAL REVIEW LETTERS, 1999, 82 (16) :3316-3319

[8] COUPLING OF AN EXCITED MOLECULE TO SURFACE PLASMONS [J].

MORAWITZ, H ;

PHILPOTT, MR .

PHYSICAL REVIEW B, 1974, 10 (12) :4863-4868

[9]

Neogi A, 2002, PHYS REV B, V66, DOI 10.1103/PhysRevB.66.153305

[10] TIME-RESOLVED VACUUM RABI OSCILLATIONS IN A SEMICONDUCTOR QUANTUM MICROCAVITY [J].

NORRIS, TB ;

RHEE, JK ;

SUNG, CY ;

ARAKAWA, Y ;

NISHIOKA, M ;

WEISBUCH, C .

PHYSICAL REVIEW B, 1994, 50 (19) :14663-14666

← 1 2 →