Novel lasing action in dye-doped polymer films coated on large pseudotabular Ag islands

被引:5
作者
Kawasaki, Mitsuo [1 ]
Mine, Shuki [1 ]
机构
[1] Kyoto Univ, Grad Sch Engn, Dept Mol Engn, Kyoto 6158510, Japan
关键词
D O I
10.1021/jp062518g
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
An similar to 15 mu m thick polymer film doped (similar to 5 mM) with a laser dye, when coated on large pseudotabular Ag islands and pumped by a nanosecond laser, generated a single sharp stimulated emission with a bandwidth down to 2.5 nm. We attribute this novel, low-threshold (similar to 1 mJ/cm(2)) lasing action to the surface-enhanced fluorescence of the dyes very near the Ag islands. This highly surface-sensitive lasing concept was supported by the fact that the lasing action was almost completely eliminated by separating the Ag islands and the dye-doped polymer film with a molecularly thin (similar to 14 angstrom) spacer.
引用
收藏
页码:15052 / 15054
页数:3
相关论文
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